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题名: Nanosized Co- and Ni-Catalyzed Ammonia Borane for Hydrogen Storage
作者: He, Teng1;  Xiong, Zhitao1;  Wu, Guotao1;  Chu, Hailiang1;  Wu, Chengzhang1;  Zhang, Tao1;  Chen, Ping1, 2, 3
通讯作者: 陈萍
刊名: CHEMISTRY OF MATERIALS
发表日期: 2009-06-09
DOI: 10.1021/cm900672h
卷: 21, 期:11, 页:2315-2318
收录类别: SCI
文章类型: Article
部门归属: 19,15
项目归属: 1901,1501
产权排名: 1;1
WOS标题词: Science & Technology ;  Physical Sciences ;  Technology
类目[WOS]: Chemistry, Physical ;  Materials Science, Multidisciplinary
研究领域[WOS]: Chemistry ;  Materials Science
英文摘要: A "co-precipitation" method was applied to introduce nanosized Co- and Ni-based catalysts to ammonia borane. It was observed that approximately 1 equiv. of hydrogen was evolved from the doped ammonia borane samples at a temperature as low as 59 degrees C. Moreover, the catalytic dehydrogenation did not present any induction period, undesirable byproduct borazine, or sample forming. Electron paramagnetic resonance (EPR) characterization revealed that Co in a partially reduced state is the active species in the catalytic dehydrogenation of ammonia borane.
关键词[WOS]: THERMAL-DECOMPOSITION ;  DEHYDROGENATION ;  COBALT ;  HYDRODESULFURIZATION ;  AMIDOBORANES ;  HYDROLYSIS ;  GENERATION ;  CHEMISTRY ;  RELEASE ;  LITHIUM
语种: 英语
原文出处: 查看原文
WOS记录号: WOS:000266708700020
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/101763
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China
2.Natl Univ Singapore, Dept Phys, Singapore 117542, Singapore
3.Natl Univ Singapore, Dept Chem, Singapore 117542, Singapore

Recommended Citation:
He, Teng,Xiong, Zhitao,Wu, Guotao,et al. Nanosized Co- and Ni-Catalyzed Ammonia Borane for Hydrogen Storage[J]. CHEMISTRY OF MATERIALS,2009,21(11):2315-2318.
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