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Characterization and Catalytic Properties of the Ni/Al2O3 Catalysts for Aqueous-phase Reforming of Glucose
Wen, Guodong1,2; Xu, Yunpeng1; Xu, Zhusheng1; Tian, Zhijian1,3; Tian ZJ(田志坚)
关键词Aqueous-phase Reforming Glucose Hydrogen Ni/al2o3
刊名CATALYSIS LETTERS
2009-04-01
DOI10.1007/s10562-008-9810-0
129期:1-2页:250-257
收录类别SCI
文章类型Article
部门归属8
项目归属802
产权排名1;1
WOS标题词Science & Technology ; Physical Sciences
类目[WOS]Chemistry, Physical
研究领域[WOS]Chemistry
关键词[WOS]BIOMASS-DERIVED HYDROCARBONS ; SUPPORTED METAL-CATALYSTS ; OXYGENATED HYDROCARBONS ; HYDROGEN-PRODUCTION ; NICKEL-CATALYSTS ; GLYCEROL ; DECOMPOSITION ; WATER ; SIZE
英文摘要Two Ni/Al2O3 catalysts with high Ni loadings of 36 wt% and 48 wt%, which possess high activities for aqueous-phase reforming of glucose, have been successfully prepared by a novel two-step impregnation method. The catalytic performance was investigated at 533 K and autogenous pressure in a batch reactor and a significant enhancement in hydrogen yield was observed over the catalyst prepared by two-step impregnation as compared to the corresponding catalyst prepared by conventional single impregnation. The catalysts were characterized by XRD, N-2 adsorption/desorption, H-2 chemisorption, O-2 uptake, TPO, H-2-TPR and TEM. It was found that two-step impregnation yielded catalysts with higher nickel dispersion as well as smaller nickel particle size compared to single impregnation.
语种英语
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WOS记录号WOS:000264318300036
引用统计
被引频次:27[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/102137
专题中国科学院大连化学物理研究所
通讯作者Tian ZJ(田志坚)
作者单位1.Chinese Acad Sci, Dalian Inst Chem Phys, Lab Appl Catalysis, Dalian 116023, Peoples R China
2.Chinese Acad Sci, Grad Univ, Beijing 100049, Peoples R China
3.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China
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GB/T 7714
Wen, Guodong,Xu, Yunpeng,Xu, Zhusheng,et al. Characterization and Catalytic Properties of the Ni/Al2O3 Catalysts for Aqueous-phase Reforming of Glucose[J]. CATALYSIS LETTERS,2009,129(1-2):250-257.
APA Wen, Guodong,Xu, Yunpeng,Xu, Zhusheng,Tian, Zhijian,&田志坚.(2009).Characterization and Catalytic Properties of the Ni/Al2O3 Catalysts for Aqueous-phase Reforming of Glucose.CATALYSIS LETTERS,129(1-2),250-257.
MLA Wen, Guodong,et al."Characterization and Catalytic Properties of the Ni/Al2O3 Catalysts for Aqueous-phase Reforming of Glucose".CATALYSIS LETTERS 129.1-2(2009):250-257.
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