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Characterization and Catalytic Properties of the Ni/Al2O3 Catalysts for Aqueous-phase Reforming of Glucose
Wen, Guodong1,2; Xu, Yunpeng1; Xu, Zhusheng1; Tian, Zhijian1,3; Tian ZJ(田志坚)
KeywordAqueous-phase Reforming Glucose Hydrogen Ni/al2o3
Source PublicationCATALYSIS LETTERS
2009-04-01
DOI10.1007/s10562-008-9810-0
Volume129Issue:1-2Pages:250-257
Indexed BySCI
SubtypeArticle
Department8
Funding Project802
Contribution Rank1;1
WOS HeadingsScience & Technology ; Physical Sciences
WOS SubjectChemistry, Physical
WOS Research AreaChemistry
WOS KeywordBIOMASS-DERIVED HYDROCARBONS ; SUPPORTED METAL-CATALYSTS ; OXYGENATED HYDROCARBONS ; HYDROGEN-PRODUCTION ; NICKEL-CATALYSTS ; GLYCEROL ; DECOMPOSITION ; WATER ; SIZE
AbstractTwo Ni/Al2O3 catalysts with high Ni loadings of 36 wt% and 48 wt%, which possess high activities for aqueous-phase reforming of glucose, have been successfully prepared by a novel two-step impregnation method. The catalytic performance was investigated at 533 K and autogenous pressure in a batch reactor and a significant enhancement in hydrogen yield was observed over the catalyst prepared by two-step impregnation as compared to the corresponding catalyst prepared by conventional single impregnation. The catalysts were characterized by XRD, N-2 adsorption/desorption, H-2 chemisorption, O-2 uptake, TPO, H-2-TPR and TEM. It was found that two-step impregnation yielded catalysts with higher nickel dispersion as well as smaller nickel particle size compared to single impregnation.
Language英语
URL查看原文
WOS IDWOS:000264318300036
Citation statistics
Cited Times:33[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/102137
Collection中国科学院大连化学物理研究所
Corresponding AuthorTian ZJ(田志坚)
Affiliation1.Chinese Acad Sci, Dalian Inst Chem Phys, Lab Appl Catalysis, Dalian 116023, Peoples R China
2.Chinese Acad Sci, Grad Univ, Beijing 100049, Peoples R China
3.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China
Recommended Citation
GB/T 7714
Wen, Guodong,Xu, Yunpeng,Xu, Zhusheng,et al. Characterization and Catalytic Properties of the Ni/Al2O3 Catalysts for Aqueous-phase Reforming of Glucose[J]. CATALYSIS LETTERS,2009,129(1-2):250-257.
APA Wen, Guodong,Xu, Yunpeng,Xu, Zhusheng,Tian, Zhijian,&田志坚.(2009).Characterization and Catalytic Properties of the Ni/Al2O3 Catalysts for Aqueous-phase Reforming of Glucose.CATALYSIS LETTERS,129(1-2),250-257.
MLA Wen, Guodong,et al."Characterization and Catalytic Properties of the Ni/Al2O3 Catalysts for Aqueous-phase Reforming of Glucose".CATALYSIS LETTERS 129.1-2(2009):250-257.
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