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Acetic Acid from the Carbonylation of Chloride Methane Over Rhodium Based Catalysts
Fan, Yafang; Ma, Ding; Bao, Xinhe; Bao XH(包信和)
关键词Methane Activation Chloride Methane Carbonylation Rhodium Catalysts
刊名CATALYSIS LETTERS
2009-07-01
DOI10.1007/s10562-009-0017-9
130期:3-4页:286-290
收录类别SCI
文章类型Article
部门归属5
项目归属502
产权排名1;1
WOS标题词Science & Technology ; Physical Sciences
类目[WOS]Chemistry, Physical
研究领域[WOS]Chemistry
关键词[WOS]CONVERSION ; HYDROLYSIS ; ACTIVATION ; CHEMISTRY ; IODIDE ; FUELS
英文摘要A new route for the indirect conversion of methane that makes use of the latest advance in methyl chloride production is reported. Acetic acid was produced from the carbonylation of methyl chloride by carbon monoxide over a variety of catalysts. The presence of promoters was crucial for the carbonylation reaction. The yield of acetic acid reached 84.7% with RhCl(3) as catalyst and PPh(3)/KI as promoters. The effects of reaction temperature, carbon monoxide pressure, and reaction time were investigated. The possible reaction mechanism was discussed.
语种英语
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WOS记录号WOS:000267330300003
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被引频次:5[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/102333
专题中国科学院大连化学物理研究所
通讯作者Bao XH(包信和)
作者单位Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China
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GB/T 7714
Fan, Yafang,Ma, Ding,Bao, Xinhe,et al. Acetic Acid from the Carbonylation of Chloride Methane Over Rhodium Based Catalysts[J]. CATALYSIS LETTERS,2009,130(3-4):286-290.
APA Fan, Yafang,Ma, Ding,Bao, Xinhe,&包信和.(2009).Acetic Acid from the Carbonylation of Chloride Methane Over Rhodium Based Catalysts.CATALYSIS LETTERS,130(3-4),286-290.
MLA Fan, Yafang,et al."Acetic Acid from the Carbonylation of Chloride Methane Over Rhodium Based Catalysts".CATALYSIS LETTERS 130.3-4(2009):286-290.
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