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题名: Acetic Acid from the Carbonylation of Chloride Methane Over Rhodium Based Catalysts
作者: Fan, Yafang1;  Ma, Ding1;  Bao, Xinhe1
通讯作者: 包信和
关键词: Methane activation ;  Chloride methane ;  Carbonylation ;  Rhodium catalysts
刊名: CATALYSIS LETTERS
发表日期: 2009-07-01
DOI: 10.1007/s10562-009-0017-9
卷: 130, 期:3-4, 页:286-290
收录类别: SCI
文章类型: Article
部门归属: 5
项目归属: 502
产权排名: 1;1
WOS标题词: Science & Technology ;  Physical Sciences
类目[WOS]: Chemistry, Physical
研究领域[WOS]: Chemistry
英文摘要: A new route for the indirect conversion of methane that makes use of the latest advance in methyl chloride production is reported. Acetic acid was produced from the carbonylation of methyl chloride by carbon monoxide over a variety of catalysts. The presence of promoters was crucial for the carbonylation reaction. The yield of acetic acid reached 84.7% with RhCl(3) as catalyst and PPh(3)/KI as promoters. The effects of reaction temperature, carbon monoxide pressure, and reaction time were investigated. The possible reaction mechanism was discussed.
关键词[WOS]: CONVERSION ;  HYDROLYSIS ;  ACTIVATION ;  CHEMISTRY ;  IODIDE ;  FUELS
语种: 英语
原文出处: 查看原文
WOS记录号: WOS:000267330300003
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/102333
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China

Recommended Citation:
Fan, Yafang,Ma, Ding,Bao, Xinhe. Acetic Acid from the Carbonylation of Chloride Methane Over Rhodium Based Catalysts[J]. CATALYSIS LETTERS,2009,130(3-4):286-290.
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