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Acetic Acid from the Carbonylation of Chloride Methane Over Rhodium Based Catalysts
Fan, Yafang; Ma, Ding; Bao, Xinhe; Bao XH(包信和)
KeywordMethane Activation Chloride Methane Carbonylation Rhodium Catalysts
Source PublicationCATALYSIS LETTERS
2009-07-01
DOI10.1007/s10562-009-0017-9
Volume130Issue:3-4Pages:286-290
Indexed BySCI
SubtypeArticle
Department5
Funding Project502
Contribution Rank1;1
WOS HeadingsScience & Technology ; Physical Sciences
WOS SubjectChemistry, Physical
WOS Research AreaChemistry
WOS KeywordCONVERSION ; HYDROLYSIS ; ACTIVATION ; CHEMISTRY ; IODIDE ; FUELS
AbstractA new route for the indirect conversion of methane that makes use of the latest advance in methyl chloride production is reported. Acetic acid was produced from the carbonylation of methyl chloride by carbon monoxide over a variety of catalysts. The presence of promoters was crucial for the carbonylation reaction. The yield of acetic acid reached 84.7% with RhCl(3) as catalyst and PPh(3)/KI as promoters. The effects of reaction temperature, carbon monoxide pressure, and reaction time were investigated. The possible reaction mechanism was discussed.
Language英语
URL查看原文
WOS IDWOS:000267330300003
Citation statistics
Cited Times:5[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/102333
Collection中国科学院大连化学物理研究所
Corresponding AuthorBao XH(包信和)
AffiliationChinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China
Recommended Citation
GB/T 7714
Fan, Yafang,Ma, Ding,Bao, Xinhe,et al. Acetic Acid from the Carbonylation of Chloride Methane Over Rhodium Based Catalysts[J]. CATALYSIS LETTERS,2009,130(3-4):286-290.
APA Fan, Yafang,Ma, Ding,Bao, Xinhe,&包信和.(2009).Acetic Acid from the Carbonylation of Chloride Methane Over Rhodium Based Catalysts.CATALYSIS LETTERS,130(3-4),286-290.
MLA Fan, Yafang,et al."Acetic Acid from the Carbonylation of Chloride Methane Over Rhodium Based Catalysts".CATALYSIS LETTERS 130.3-4(2009):286-290.
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