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A promotion effect of alkaline-earth chloride on N-hydroxyphthalimide-catalyzed aerobic oxidation of hydrocarbons
Yang, Xiaomei1; Zhou, Lipeng1; Chen, Yong1; Chen, Chen2; Su, Yunlai1; Miao, Hong2; Xu, Jie2; Xu J(徐杰)
关键词Alkaline-earth Chloride N-hydroxyphthalimide Aerobic Oxidation Hydrocarbons
刊名CATALYSIS COMMUNICATIONS
2009-11-25
DOI10.1016/j.catcom.2009.09.019
11期:3页:171-174
收录类别SCI ; CCR
文章类型Article
部门归属2
项目归属204
产权排名2;4
WOS标题词Science & Technology ; Physical Sciences
类目[WOS]Chemistry, Physical
研究领域[WOS]Chemistry
关键词[WOS]MOLECULAR-OXYGEN ; NITROXYL RADICALS ; ORGANIC-COMPOUNDS ; DIOXYGEN ; ALCOHOLS ; BROMIDE ; NHPI
英文摘要Alkaline-earth chloride was used as an effective promoter for the aerobic oxidation of hydrocarbons catalyzed by N-hydroxyphthalimide (NHPI). Various hydrocarbons including benzylic compounds, cycloalkene, and cycloalkane can be easily oxygenated with molecular oxygen catalyzed by the alkaline-earth chloride/NHPI system. Ultraviolet-visible (UV-vis) spectroscopy and Fourier transform infrared (FT-IR) spectroscopy were employed to investigate the essential of the promotion effect of alkaline-earth chloride. The results revealed that alkaline-earth chloride facilitated the generation of the active species phthalimide-N-oxyl (PINO) radical which further catalyzed the oxidation of hydrocarbons. (C) 2009 Elsevier B.V. All rights reserved.
语种英语
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WOS记录号WOS:000272833900007
引用统计
被引频次:23[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/102669
专题中国科学院大连化学物理研究所
通讯作者Xu J(徐杰)
作者单位1.Zhengzhou Univ, Dept Chem, Zhengzhou 450001, Peoples R China
2.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China
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GB/T 7714
Yang, Xiaomei,Zhou, Lipeng,Chen, Yong,et al. A promotion effect of alkaline-earth chloride on N-hydroxyphthalimide-catalyzed aerobic oxidation of hydrocarbons[J]. CATALYSIS COMMUNICATIONS,2009,11(3):171-174.
APA Yang, Xiaomei.,Zhou, Lipeng.,Chen, Yong.,Chen, Chen.,Su, Yunlai.,...&徐杰.(2009).A promotion effect of alkaline-earth chloride on N-hydroxyphthalimide-catalyzed aerobic oxidation of hydrocarbons.CATALYSIS COMMUNICATIONS,11(3),171-174.
MLA Yang, Xiaomei,et al."A promotion effect of alkaline-earth chloride on N-hydroxyphthalimide-catalyzed aerobic oxidation of hydrocarbons".CATALYSIS COMMUNICATIONS 11.3(2009):171-174.
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