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题名: Iron Chloride/4-Acetamido-TEMPO/Sodium Nitrite-Catalyzed Aerobic Oxidation of Primary Alcohols to the Aldehydes
作者: Yin, Weili1;  Chu, Changhu1;  Lu, Qiongqiong1;  Tao, Jianwei1;  Liang, Xinmiao1, 2;  Liu, Renhua1
通讯作者: 梁鑫淼 ;  刘仁华
关键词: aerobic oxidation ;  iron chloride ;  primary alcohols ;  sodium nitrite ;  TEMPO
刊名: ADVANCED SYNTHESIS & CATALYSIS
发表日期: 2010
DOI: 10.1002/adsc.200900662
卷: 352, 期:1, 页:113-118
收录类别: SCI ;  IC ;  CCR
文章类型: Article
部门归属: 18
项目归属: 1803
产权排名: 2;5
WOS标题词: Science & Technology ;  Physical Sciences
类目[WOS]: Chemistry, Applied ;  Chemistry, Organic
研究领域[WOS]: Chemistry
英文摘要: A variety of 4-substituted 2,2,6,6-tetramethylpiperidyl-1-oxy (TEMPO) derivatives has been screened for their ability in the oxidation of primary alcohols to the aldehydes with dioxygen under mild conditions. An evaluation of the efficiency of these 4-substituted TEMPO derivatives in the alcohol oxidation may allow an insight into the effect of the structural variations of TEMPO on the oxidation of alcohols, which should facilitate catalyst design and screening efforts. Based on the screening results of 4-substituted TEMPO derivatives, the catalyst comprised of 4-acetamido-TEMPO, iron chloride and sodium nitrite, has been developed for the highly efficient oxidation of a wide range of primary alcohols including primary aliphatic alcohols to the corresponding aldehydes under mild conditions.
关键词[WOS]: TRANSITION-METAL-FREE ;  AQUEOUS HYDROGEN-PEROXIDE ;  LIQUID-PHASE OXIDATION ;  MOLECULAR-OXYGEN ;  MILD CONDITIONS ;  SELECTIVE OXIDATION ;  BENZYLIC ALCOHOLS ;  PALLADIUM NANOPARTICLES ;  ATMOSPHERIC OXYGEN ;  RUTHENIUM CATALYST
语种: 英语
原文出处: 查看原文
WOS记录号: WOS:000274339500009
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/103075
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.E China Univ Sci & Technol, Sch Pharm, Shanghai 200237, Peoples R China
2.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China

Recommended Citation:
Yin, Weili,Chu, Changhu,Lu, Qiongqiong,et al. Iron Chloride/4-Acetamido-TEMPO/Sodium Nitrite-Catalyzed Aerobic Oxidation of Primary Alcohols to the Aldehydes[J]. ADVANCED SYNTHESIS & CATALYSIS,2010,352(1):113-118.
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