DICP OpenIR
学科主题物理化学
Reactions and carbide formation on thin Pd membranes during separation of CH4/H2 and CO/H2 mixtures in the limit of maximum H2 extraction
Li H(李慧); A.Goldbach; Xu HY(徐恒泳); Li WZ(李文钊)
会议名称10th International Conference on Inorganic Membranes
会议日期2008-8-18
2008-08-18
会议地点日本
页码106/2
部门归属八室
主办者日本膜协会和早稻田大学
英文摘要Inhibitive effects of CO and CH4 on H2 permeation through 2-3 μm thick Pd membranes were studied by comparing their impact to that of inert N2. CO lead to reduction of the H2 permeance at all temperatures while it increased in the presence of CH4. Below 623 K CO adsorption was the main reason for the decrease of H2 permeation while carbon deposition due to CO decomposition became important at higher temperatures. The larger H2 fluxes from mixtures with CH4 resulted from decomposition of that hydrocarbon, leading to carbonaceous phases above 723 K. Apparently the presence of 50% H2 cannot completely suppress carbon deposition from CO at elevated temperatures.
语种中文
文献类型会议论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/113450
专题中国科学院大连化学物理研究所
通讯作者Xu HY(徐恒泳)
推荐引用方式
GB/T 7714
Li H,A.Goldbach,Xu HY,et al. Reactions and carbide formation on thin Pd membranes during separation of CH4/H2 and CO/H2 mixtures in the limit of maximum H2 extraction[C],2008:106/2.
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