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学科主题物理化学
Insight into the phase evolution of iron phosphate catalyst during the oxidative bromination of methane
Lin RH(林荣和); Ding YJ(丁云杰); Gong LF(龚磊峰); Chen WM(陈维苗); Yan L(严丽); Lv Y(吕元)
会议名称Sixth Tokyo Conference on Advanced Catalytic Science and Technology & Fifth Asia Pacific Congress on Catalysis
会议日期2010-7-18
2010-07-18
会议地点日本
页码118/2
部门归属八室
主办者Catalysis Society of Japan
英文摘要FePO4/SiO2,as an inexpensive and widely used material, was firstly employed for the oxidative bromination of methane, which showed effective and stable performance at 570℃, namely, 49% methane conversion and 95% total selectivity for CH3Br/CO(CH3Br:CO ≈1)were obtained on a single pass. The products could be directly used as a feedstock for the manufacture of acetic acid. 57Fe Mossbauer spectroscopic studies revealed that the FePO4 components of the fresh catalyst transformed quickly into stable active species during the induction period, and the active components of the stable catalyst have been found to consist of near-equimolar α-Fe3(P2O7)2 and Fe2P2O7.
语种中文
文献类型会议论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/114504
专题中国科学院大连化学物理研究所
通讯作者Ding YJ(丁云杰)
推荐引用方式
GB/T 7714
Lin RH,Ding YJ,Gong LF,et al. Insight into the phase evolution of iron phosphate catalyst during the oxidative bromination of methane[C],2010:118/2.
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