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学科主题物理化学
Phosphotungstic Acid Encapsulated in Metal-Organic Framework as Catalysts for Carbohydrate Dehydration to 5-Hydroxymethylfurfural
Zhang, Yanmei1,2; Degirmenci, Volkan2; Li, Can1; Hensen, Emiel J. M.2; Li C(李灿); EmielJ.M.Hensen
关键词Biomass Carbohydrates Heterogeneous Catalysis Metal-organic Frameworks Solid Acids
刊名CHEMSUSCHEM
2011
ISSN待补充
DOI10.1002/cssc.201000284
4期:1页:59-64
收录类别SCI
文章类型Article
部门归属5
项目归属503
产权排名1,1
WOS标题词Science & Technology ; Physical Sciences
类目[WOS]Chemistry, Multidisciplinary
研究领域[WOS]Chemistry
关键词[WOS]MESOPOROUS SILICA ; HYDROGEN STORAGE ; DRUG-DELIVERY ; SURFACE-AREA ; IONIC LIQUID ; GIANT PORES ; D-FRUCTOSE ; BIOMASS ; SITES ; OXIDATION
英文摘要Phosphotungstic Acid Encapsulated in Metal-Organic Framework as Catalysts for Carbohydrate Dehydration to 5-Hydroxymethylfurfural; MIL-101, a chromium-based metal-organic framework, is known for its very large pore size, large surface area and good stability. However, applications of this material in catalysis are still limited. 5-Hydroxymethylfurfural (HMF) has been considered a renewable chemical platform for the production of liquid fuels and fine chemicals. Phosphotungstic acid, H(3)PW(12)O(40) (PTA), encapsulated in MIL-101 is evaluated as a potential catalyst for the selective dehydration of fructose and glucose to 5-hydroxymethylfurfural. The results demonstrate that PTA/MIL-101 is effective for HMF production from fructose in DMSO and can be reused. This is the first example of the application of a metal-organic framework in carbohydrate dehydration.
语种英语
WOS记录号WOS:000287138900010
引用统计
被引频次:128[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/115742
专题中国科学院大连化学物理研究所
通讯作者Li C(李灿); EmielJ.M.Hensen
作者单位1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China
2.Eindhoven Univ Technol, Schuit Inst Catalysis, NL-5600 MB Eindhoven, Netherlands
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Zhang, Yanmei,Degirmenci, Volkan,Li, Can,et al. Phosphotungstic Acid Encapsulated in Metal-Organic Framework as Catalysts for Carbohydrate Dehydration to 5-Hydroxymethylfurfural[J]. CHEMSUSCHEM,2011,4(1):59-64.
APA Zhang, Yanmei,Degirmenci, Volkan,Li, Can,Hensen, Emiel J. M.,李灿,&EmielJ.M.Hensen.(2011).Phosphotungstic Acid Encapsulated in Metal-Organic Framework as Catalysts for Carbohydrate Dehydration to 5-Hydroxymethylfurfural.CHEMSUSCHEM,4(1),59-64.
MLA Zhang, Yanmei,et al."Phosphotungstic Acid Encapsulated in Metal-Organic Framework as Catalysts for Carbohydrate Dehydration to 5-Hydroxymethylfurfural".CHEMSUSCHEM 4.1(2011):59-64.
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