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学科主题物理化学
Synthesis, Crystal Structures, and Luminescence and Magnetic Properties of 3D Chiral and Achiral Lanthanide Diphosphonates Containing Left- and Right-Handed Helical Chains
Dong, Da-Peng1; Liu, Lei1; Sun, Zhen-Gang1; Jiao, Cheng-Qi1; Liu, Zhong-Min2; Li, Chao1; Zhu, Yan-Yu1; Chen, Kai1; Wang, Cheng-Lin1; Zhen-GangSun
刊名CRYSTAL GROWTH & DESIGN
2011-12-01
ISSN待补充
DOI10.1021/cg2009368
11期:12页:5346-5354
收录类别SCI
文章类型Article
部门归属DNL12
项目归属DNL12
产权排名2,5
WOS标题词Science & Technology ; Physical Sciences ; Technology
类目[WOS]Chemistry, Multidisciplinary ; Crystallography ; Materials Science, Multidisciplinary
研究领域[WOS]Chemistry ; Crystallography ; Materials Science
关键词[WOS]METAL PHOSPHONATE CHEMISTRY ; CARBOXYLATE-PHOSPHONATES ; COORDINATION POLYMERS ; SPONTANEOUS RESOLUTION ; ORGANIC FRAMEWORK ; BUILDING-BLOCKS ; POROUS SOLIDS ; ZEOLITE-TYPE ; SERIES ; STATE
英文摘要Synthesis, Crystal Structures, and Luminescence and Magnetic Properties of 3D Chiral and Achiral Lanthanide Diphosphonates Containing Left- and Right-Handed Helical Chains; Using the heptadentate ligand hedpH(4) (1-hydroxyethylidenediphosphonic acid) and lanthanide chloride, two isomorphous series of coordination frameworks of the general formula [NH4] [Ln(hedp)(H2O)]center dot H2O (series 1, orthorhombic P2(1)2(1)2(1), Ln = La (1), Ce (2), Pr (3), Nd (4)) and [NH4] [Ln(hedp)(H2O)] (series 2, orthorhombic Pnma, Ln = Sm (5), Eu (6), Gd (7), Tb (8), Dy (9), Y (10), Er (11)) have been assembled and characterized with IR, elemental analysis, thermogravimetric analysis, and single-crystal and powder X-ray diffraction methods. In both series, each inorganic chain based on LnO(8) and CPO3 polyhedra are interconnected through phosphonate ligands to form chiral and achiral 3D open-framework structures with left- and right-handed helical chains. Meanwhile, the two series also exhibit two types of 3D framework structures with similar network topologies. The crystal water molecule plays an important role to induce chiral structure and affects the crystal packing of the molecules with extensive hydrogen bonding. The luminescence properties of compounds 5, 6, 8 and 9 and the magnetic property of compound 7 have also been studied.
语种英语
WOS记录号WOS:000297609100024
引用统计
被引频次:43[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/115851
专题中国科学院大连化学物理研究所
通讯作者Zhen-GangSun
作者单位1.Liaoning Normal Univ, Sch Chem & Chem Engn, Inst Chem Functionalized Mat, Dalian 116029, Peoples R China
2.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China
推荐引用方式
GB/T 7714
Dong, Da-Peng,Liu, Lei,Sun, Zhen-Gang,et al. Synthesis, Crystal Structures, and Luminescence and Magnetic Properties of 3D Chiral and Achiral Lanthanide Diphosphonates Containing Left- and Right-Handed Helical Chains[J]. CRYSTAL GROWTH & DESIGN,2011,11(12):5346-5354.
APA Dong, Da-Peng.,Liu, Lei.,Sun, Zhen-Gang.,Jiao, Cheng-Qi.,Liu, Zhong-Min.,...&Zhen-GangSun.(2011).Synthesis, Crystal Structures, and Luminescence and Magnetic Properties of 3D Chiral and Achiral Lanthanide Diphosphonates Containing Left- and Right-Handed Helical Chains.CRYSTAL GROWTH & DESIGN,11(12),5346-5354.
MLA Dong, Da-Peng,et al."Synthesis, Crystal Structures, and Luminescence and Magnetic Properties of 3D Chiral and Achiral Lanthanide Diphosphonates Containing Left- and Right-Handed Helical Chains".CRYSTAL GROWTH & DESIGN 11.12(2011):5346-5354.
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