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学科主题物理化学
Highly Efficient Pumping of Vibrationally Excited HD Molecules via Stark-Induced Adiabatic Raman Passage
Wang, Tao1; Yang, Tiangang1,2; Xiao, Chunlei1; Dai, Dongxu1; Yang, Xueming1; Xiao CL(肖春雷); Yang XM(杨学明)
刊名JOURNAL OF PHYSICAL CHEMISTRY LETTERS
2013-02-07
DOI10.1021/jz302103u
4期:3页:368-371
收录类别SCI
文章类型Article
部门归属11
项目归属1102
产权排名1,1
WOS标题词Science & Technology ; Physical Sciences ; Technology
类目[WOS]Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Atomic, Molecular & Chemical
研究领域[WOS]Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics
关键词[WOS]POPULATION TRANSFER ; CROSS-SECTIONS ; DYNAMICS
英文摘要A primary prerequisite to study reactivity of vibrationally excited species is to efficiently prepare reacting species in a well-defined vibrational level. Efficient pumping of IR active vibrational modes in a molecule can be achieved by direct IR absorption. For vibrational modes that are only Raman active, however, efficient preparation of vibrationally excited states in those modes is not easily attainable. In this work, we have shown that highly efficient preparation of the HD(v = 1) state using the Stark-induced adiabatic Raman passage (SARI?) scheme is feasible. As high as 91% population transfer from v = 0 to 1 of HD has been demonstrated in our experiment. This method provides new opportunities for future experimental studies on the dynamics of vibrational state molecules, especially H-2, in both gas-phase and beam-surface reactions.
语种英语
WOS记录号WOS:000314907500005
引用统计
被引频次:10[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/117653
专题中国科学院大连化学物理研究所
通讯作者Xiao CL(肖春雷); Yang XM(杨学明)
作者单位1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China
2.Dalian Univ Technol, Sch Phys & Optoelect Engn, Dalian 116023, Liaoning, Peoples R China
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GB/T 7714
Wang, Tao,Yang, Tiangang,Xiao, Chunlei,et al. Highly Efficient Pumping of Vibrationally Excited HD Molecules via Stark-Induced Adiabatic Raman Passage[J]. JOURNAL OF PHYSICAL CHEMISTRY LETTERS,2013,4(3):368-371.
APA Wang, Tao.,Yang, Tiangang.,Xiao, Chunlei.,Dai, Dongxu.,Yang, Xueming.,...&杨学明.(2013).Highly Efficient Pumping of Vibrationally Excited HD Molecules via Stark-Induced Adiabatic Raman Passage.JOURNAL OF PHYSICAL CHEMISTRY LETTERS,4(3),368-371.
MLA Wang, Tao,et al."Highly Efficient Pumping of Vibrationally Excited HD Molecules via Stark-Induced Adiabatic Raman Passage".JOURNAL OF PHYSICAL CHEMISTRY LETTERS 4.3(2013):368-371.
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