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学科主题物理化学
New chiral ferrocenyl P,S-ligands for highly diastereo- and enantioselective Ag(I)-catalyzed asymmetric [3+2] cycloaddition of azomethine ylides
Han, Mei-Ling1,2; Wang, Dao-Yong1; Zeng, Pei-Wei1; Zheng, Zhuo1; Hu, Xiang-Ping1; Hu XP(胡向平)
刊名TETRAHEDRON-ASYMMETRY
2012-02-29
DOI10.1016/j.tetasy.2012.02.017
23期:3-4页:306-312
收录类别SCI ; IC ; CCR
文章类型Article
部门归属2
项目归属02T2
产权排名2,1
类目[WOS]Chemistry, Inorganic & Nuclear ; Chemistry, Organic ; Chemistry, Physical
研究领域[WOS]Chemistry
关键词[WOS]1,3-DIPOLAR CYCLOADDITION ; DIPHOSPHINE LIGANDS ; ALLYLIC ALKYLATIONS ; HYDROGENATION ; CATALYSIS ; DERIVATIVES ; REACTIVITY ; COMPLEX ; ENONES ; FAMILY
英文摘要A new family of chiral ferrocenyl P,S-ligands incorporating an indole ring at the alpha-ferrocenylmethyl position has been prepared via a Friedel-Crafts alkylation reaction of (R-c,S-Fc)-PPFA with a variety of 2-indole thioethers. These newly developed ferrocenyl P,S-ligands proved to be efficient in the AgOAc-catalyzed asymmetric [3+2] cycloaddition of azomethine ylides with various dipolarophiles, giving cycloadducts with high diastereoselectivities and enantioselectivities (up to 99% ee). (C) 2012 Elsevier Ltd. All rights reserved.
语种英语
WOS记录号WOS:000302973900018
引用统计
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/117906
专题中国科学院大连化学物理研究所
通讯作者Hu XP(胡向平)
作者单位1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China
2.Tianjin Univ, Sch Chem Engn & Technol, Tianjin 300072, Peoples R China
推荐引用方式
GB/T 7714
Han, Mei-Ling,Wang, Dao-Yong,Zeng, Pei-Wei,et al. New chiral ferrocenyl P,S-ligands for highly diastereo- and enantioselective Ag(I)-catalyzed asymmetric [3+2] cycloaddition of azomethine ylides[J]. TETRAHEDRON-ASYMMETRY,2012,23(3-4):306-312.
APA Han, Mei-Ling,Wang, Dao-Yong,Zeng, Pei-Wei,Zheng, Zhuo,Hu, Xiang-Ping,&胡向平.(2012).New chiral ferrocenyl P,S-ligands for highly diastereo- and enantioselective Ag(I)-catalyzed asymmetric [3+2] cycloaddition of azomethine ylides.TETRAHEDRON-ASYMMETRY,23(3-4),306-312.
MLA Han, Mei-Ling,et al."New chiral ferrocenyl P,S-ligands for highly diastereo- and enantioselective Ag(I)-catalyzed asymmetric [3+2] cycloaddition of azomethine ylides".TETRAHEDRON-ASYMMETRY 23.3-4(2012):306-312.
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