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学科主题物理化学
The copolymerization reactivity of diols with 2,5-furandicarboxylic acid for furan-based copolyester materials
Ma, Jiping1,2,3; Pang, Yi1; Wang, Min2,3; Xu, Jie2; Ma, Hong2; Nie, Xin2; Xu J(徐杰)
刊名JOURNAL OF MATERIALS CHEMISTRY
2012
DOI10.1039/c2jm15457a
22期:8页:3457-3461
收录类别SCI
文章类型Article
部门归属DNL06
项目归属601
产权排名2,1
WOS标题词Science & Technology ; Physical Sciences ; Technology
类目[WOS]Chemistry, Physical ; Materials Science, Multidisciplinary
研究领域[WOS]Chemistry ; Materials Science
关键词[WOS]AEROBIC OXIDATION ; COMONOMER REACTIVITY ; EFFICIENT ; GLYCEROL ; CATALYST ; 2,5-DIFORMYLFURAN ; HYDROGENOLYSIS ; DEHYDRATION ; POLYESTER ; CHEMICALS
英文摘要Furan-based copolyesters were synthesized via polytransesterification of 2,5-furandicarboxylic acid (FDCA) with ethylene glycol (EG) and 1,4-butylene glycol (BG). The composition and thermal properties of the obtained copolyesters were characterized in detail by H-1 NMR and elemental analysis, differential scanning calorimeters (DSC) and thermogravimetric analysis (TGA). The H-1 NMR results showed that the ethylene segment content was consistently lower than that of butylene in the obtained copolyesters in comparison with the comonomer feeds. The reactivities of EG and BG with FDCA were intensively investigated. On the basis of kinetic studies, EG was found to be less reactive than BG. The thermal properties of the obtained copolyesters could be adjusted by variation of the EG/BG molar ratios in the copolyesters.
语种英语
WOS记录号WOS:000299695400028
引用统计
被引频次:104[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/117911
专题中国科学院大连化学物理研究所
通讯作者Xu J(徐杰)
作者单位1.Univ Akron, Dept Chem, Akron, OH 44325 USA
2.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian Natl Lab Clean Energy, Dalian 116023, Peoples R China
3.Chinese Acad Sci, Grad Univ, Beijing 100039, Peoples R China
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GB/T 7714
Ma, Jiping,Pang, Yi,Wang, Min,et al. The copolymerization reactivity of diols with 2,5-furandicarboxylic acid for furan-based copolyester materials[J]. JOURNAL OF MATERIALS CHEMISTRY,2012,22(8):3457-3461.
APA Ma, Jiping.,Pang, Yi.,Wang, Min.,Xu, Jie.,Ma, Hong.,...&徐杰.(2012).The copolymerization reactivity of diols with 2,5-furandicarboxylic acid for furan-based copolyester materials.JOURNAL OF MATERIALS CHEMISTRY,22(8),3457-3461.
MLA Ma, Jiping,et al."The copolymerization reactivity of diols with 2,5-furandicarboxylic acid for furan-based copolyester materials".JOURNAL OF MATERIALS CHEMISTRY 22.8(2012):3457-3461.
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