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学科主题物理化学
Copper(II)-Mediated Dehydrogenative Cross-Coupling of Heteroarenes
Mao, Zhifeng1; Wang, Zhe2; Xu, Zhaoqing1,2; Huang, Fei1; Yu, Zhengkun1; Wang, Rui2; Xu ZQ(许兆青); Yu ZK(余正坤); RuiWang
刊名ORGANIC LETTERS
2012-08-03
DOI10.1021/ol301517y
14期:15页:3854-3857
收录类别SCI ; IC ; CCR
文章类型Article
部门归属2
项目归属203
产权排名1,1
WOS标题词Science & Technology ; Physical Sciences
类目[WOS]Chemistry, Organic
研究领域[WOS]Chemistry
关键词[WOS]C-H BONDS ; COPPER-CATALYZED ARYLATION ; GENERAL-METHOD ; ARYL BROMIDES ; SOLE OXIDANT ; PALLADIUM ; AZOLES ; FUNCTIONALIZATIONS ; HETEROCYCLES ; ACIDS
英文摘要Cu(OAc)(2)-mediated dehydrogenative cross-coupling between two heteroarenes has been realized in the absence of any other additive. A mechanism involving a formal Cu(II) to Cu(0) route by convergent disproportionation of the copper mediator is proposed and has been evidenced by copper mirror formation during the reaction. This synthetic protocol provides a concise and "green" access to unsymmetrical biheteroarenes bearing structural motifs of substantial utility in organic synthesis.
语种英语
WOS记录号WOS:000307041600011
引用统计
被引频次:63[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/118247
专题中国科学院大连化学物理研究所
通讯作者Xu ZQ(许兆青); Yu ZK(余正坤); RuiWang
作者单位1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China
2.Lanzhou Univ, Key Lab Preclin Study New Drugs Gansu Prov, Lanzhou 730000, Peoples R China
推荐引用方式
GB/T 7714
Mao, Zhifeng,Wang, Zhe,Xu, Zhaoqing,et al. Copper(II)-Mediated Dehydrogenative Cross-Coupling of Heteroarenes[J]. ORGANIC LETTERS,2012,14(15):3854-3857.
APA Mao, Zhifeng.,Wang, Zhe.,Xu, Zhaoqing.,Huang, Fei.,Yu, Zhengkun.,...&RuiWang.(2012).Copper(II)-Mediated Dehydrogenative Cross-Coupling of Heteroarenes.ORGANIC LETTERS,14(15),3854-3857.
MLA Mao, Zhifeng,et al."Copper(II)-Mediated Dehydrogenative Cross-Coupling of Heteroarenes".ORGANIC LETTERS 14.15(2012):3854-3857.
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