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学科主题: 物理化学
题名: Surface photochemistry probed by two-photon photoemission spectroscopy
作者: Zhou, Chuanyao1;  Ma, Zhibo1;  Ren, Zefeng1;  Wodtke, Alec M.2, 3, 5;  Yang, Xueming1, 2, 4, 5
通讯作者: 杨学明
刊名: ENERGY & ENVIRONMENTAL SCIENCE
发表日期: 2012-05-01
DOI: 10.1039/c2ee21493h
卷: 5, 期:5, 页:6833-6844
收录类别: SCI
文章类型: Review
部门归属: 11
项目归属: 1102
产权排名: 1,1
WOS标题词: Science & Technology ;  Physical Sciences ;  Technology ;  Life Sciences & Biomedicine
类目[WOS]: Chemistry, Multidisciplinary ;  Energy & Fuels ;  Engineering, Chemical ;  Environmental Sciences
研究领域[WOS]: Chemistry ;  Energy & Fuels ;  Engineering ;  Environmental Sciences & Ecology
英文摘要: Two-photon photoemission (2PPE) has been widely used in the study of electronic structure and dynamics of unoccupied electronic states on different types of surfaces and interfaces. Since 2PPE probes electronically excited states, it should be sensitive to surface excited electronic structure changes that accompany surface chemical reactions. Therefore, this method could potentially be used to study the kinetics and dynamics of surface chemical reactions as well as surface photocatalysis. In this article, we briefly review recent progress made in the study of surface photochemistry and photocatalysis using the time-dependent 2PPE (TD-2PPE) method. A few examples are given to demonstrate the application of this method in probing surface photochemistry and photocatalysis, particularly photocatalysis of methanol on TiO2 surfaces. Since many problems associated with surface photochemistry and surface photocatalysis are related to energy and environmental issues, the 2PPE technique could have important applications in the study of the fundamental problems in energy and environmental sciences.
关键词[WOS]: TERT-BUTYL-AZOBENZENE ;  MOLECULE-METAL INTERFACES ;  TO-STATE DYNAMICS ;  RUTILE TIO2(110) ;  HYDROGEN-PRODUCTION ;  ELECTRON DYNAMICS ;  TIO2 110 ;  OXYGEN-CHEMISORPTION ;  CHEMICAL-REACTIONS ;  EXCESS ELECTRONS
语种: 英语
WOS记录号: WOS:000303251500015
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/118286
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Liaoning, Peoples R China
2.Univ Gottingen, Inst Phys Chem, D-37073 Gottingen, Germany
3.Max Planck Inst Stromungsforsch, D-37073 Gottingen, Germany
4.Acad Sinica, Inst Atom & Mol Sci, Taipei, Taiwan
5.Max Planck Inst Biophys Chem, D-37073 Gottingen, Germany

Recommended Citation:
Zhou, Chuanyao,Ma, Zhibo,Ren, Zefeng,et al. Surface photochemistry probed by two-photon photoemission spectroscopy[J]. ENERGY & ENVIRONMENTAL SCIENCE,2012,5(5):6833-6844.
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