DICP OpenIR
Subject Area物理化学
Surface photochemistry probed by two-photon photoemission spectroscopy
Zhou, Chuanyao1; Ma, Zhibo1; Ren, Zefeng1; Wodtke, Alec M.2,3,5; Yang, Xueming1,2,4,5; Yang XM(杨学明)
Source PublicationENERGY & ENVIRONMENTAL SCIENCE
2012-05-01
DOI10.1039/c2ee21493h
Volume5Issue:5Pages:6833-6844
Indexed BySCI
SubtypeReview
Department11
Funding Project1102
Contribution Rank1,1
WOS HeadingsScience & Technology ; Physical Sciences ; Technology ; Life Sciences & Biomedicine
WOS SubjectChemistry, Multidisciplinary ; Energy & Fuels ; Engineering, Chemical ; Environmental Sciences
WOS Research AreaChemistry ; Energy & Fuels ; Engineering ; Environmental Sciences & Ecology
WOS KeywordTERT-BUTYL-AZOBENZENE ; MOLECULE-METAL INTERFACES ; TO-STATE DYNAMICS ; RUTILE TIO2(110) ; HYDROGEN-PRODUCTION ; ELECTRON DYNAMICS ; TIO2 110 ; OXYGEN-CHEMISORPTION ; CHEMICAL-REACTIONS ; EXCESS ELECTRONS
AbstractTwo-photon photoemission (2PPE) has been widely used in the study of electronic structure and dynamics of unoccupied electronic states on different types of surfaces and interfaces. Since 2PPE probes electronically excited states, it should be sensitive to surface excited electronic structure changes that accompany surface chemical reactions. Therefore, this method could potentially be used to study the kinetics and dynamics of surface chemical reactions as well as surface photocatalysis. In this article, we briefly review recent progress made in the study of surface photochemistry and photocatalysis using the time-dependent 2PPE (TD-2PPE) method. A few examples are given to demonstrate the application of this method in probing surface photochemistry and photocatalysis, particularly photocatalysis of methanol on TiO2 surfaces. Since many problems associated with surface photochemistry and surface photocatalysis are related to energy and environmental issues, the 2PPE technique could have important applications in the study of the fundamental problems in energy and environmental sciences.
Language英语
WOS IDWOS:000303251500015
Citation statistics
Cited Times:26[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/118286
Collection中国科学院大连化学物理研究所
Corresponding AuthorYang XM(杨学明)
Affiliation1.Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Liaoning, Peoples R China
2.Univ Gottingen, Inst Phys Chem, D-37073 Gottingen, Germany
3.Max Planck Inst Stromungsforsch, D-37073 Gottingen, Germany
4.Acad Sinica, Inst Atom & Mol Sci, Taipei, Taiwan
5.Max Planck Inst Biophys Chem, D-37073 Gottingen, Germany
Recommended Citation
GB/T 7714
Zhou, Chuanyao,Ma, Zhibo,Ren, Zefeng,et al. Surface photochemistry probed by two-photon photoemission spectroscopy[J]. ENERGY & ENVIRONMENTAL SCIENCE,2012,5(5):6833-6844.
APA Zhou, Chuanyao,Ma, Zhibo,Ren, Zefeng,Wodtke, Alec M.,Yang, Xueming,&杨学明.(2012).Surface photochemistry probed by two-photon photoemission spectroscopy.ENERGY & ENVIRONMENTAL SCIENCE,5(5),6833-6844.
MLA Zhou, Chuanyao,et al."Surface photochemistry probed by two-photon photoemission spectroscopy".ENERGY & ENVIRONMENTAL SCIENCE 5.5(2012):6833-6844.
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