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学科主题: 物理化学
题名: Organocatalytic Asymmetric 1,4-Addition of Aldehydes to Acridiniums Catalyzed by a Diarylprolinol Silyl Ether
作者: Liang, Tao1, 2;  Xiao, Jian1;  Xiong, Zhiyi1;  Li, Xingwei1
通讯作者: 肖建 ;  李兴伟
刊名: JOURNAL OF ORGANIC CHEMISTRY
发表日期: 2012-04-06
DOI: 10.1021/jo2025114
卷: 77, 期:7, 页:3583-3588
收录类别: SCI ;  IC ;  CCR
文章类型: Article
部门归属: 2
项目归属: 02T3
产权排名: 1,1
WOS标题词: Science & Technology ;  Physical Sciences
类目[WOS]: Chemistry, Organic
研究领域[WOS]: Chemistry
英文摘要: The organocatalytic enantioselective 1,4-addition of aldehydes to acridiniums catalyzed by diarylprolinol silyl ether was achieved to furnish chiral acridanes in both high yields (82-96%) and excellent enantioselectivities (up to 99% ee), which also provides the highly enantioselective intermolecular alpha-alkylation of aldehydes with acridiniums salt.
关键词[WOS]: INTERMOLECULAR ALPHA-ALKYLATION ;  MICHAEL ADDITION ;  DERIVATIVES ;  FUNCTIONALIZATION ;  NITROALKENES ;  ACTIVATION ;  EFFICIENCY ;  ALKALOIDS ;  CHEMISTRY ;  ALCOHOLS
语种: 英语
WOS记录号: WOS:000302388000063
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/118400
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China
2.NE Forestry Univ, Key Lab Biobased Mat Sci & Technol, Minist Educ, Harbin 150040, Peoples R China

Recommended Citation:
Liang, Tao,Xiao, Jian,Xiong, Zhiyi,et al. Organocatalytic Asymmetric 1,4-Addition of Aldehydes to Acridiniums Catalyzed by a Diarylprolinol Silyl Ether[J]. JOURNAL OF ORGANIC CHEMISTRY,2012,77(7):3583-3588.
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