DICP OpenIR
Subject Area物理化学
Capture and conversion of CO2 at ambient conditions by a conjugated microporous polymer
Xie, Yong1,2; Wang, Ting-Ting1; Liu, Xiao-Huan1; Zou, Kun2; Deng, Wei-Qiao1; Deng WQ(邓伟侨)
Source PublicationNATURE COMMUNICATIONS
2013-06-01
ISSN2041-1723
DOI10.1038/ncomms2960
Volume4Pages:1960
Indexed BySCI
Cooperation Status
SubtypeArticle
Department11
Funding Project11T4
Contribution Rank待补充
WOS HeadingsScience & Technology
Funding Organization1,1 ; 1,1 ; 1,1 ; 1,1
WOS SubjectMultidisciplinary Sciences
WOS Research AreaScience & Technology - Other Topics
WOS KeywordMETAL-ORGANIC FRAMEWORKS ; CARBON-DIOXIDE ; SURFACE-AREA ; CYCLIC CARBONATES ; HYDROGEN STORAGE ; CATALYSTS ; COMPLEXES ; EPOXIDES ; COPOLYMERIZATION ; NETWORKS
AbstractConjugated microporous polymers are a new class of porous materials with an extended pi-conjugation in an amorphous organic framework. Owing to the wide-ranging flexibility in the choice and design of components and the available control of pore parameters, these polymers can be tailored for use in various applications, such as gas storage, electronics and catalysis. Here we report a class of cobalt/aluminium-coordinated conjugated microporous polymers that exhibit outstanding CO2 capture and conversion performance at atmospheric pressure and room temperature. These polymers can store CO2 with adsorption capacities comparable to metal-organic frameworks. The cobalt-coordinated conjugated microporous polymers can also simultaneously function as heterogeneous catalysts for the reaction of CO2 and propylene oxide at atmospheric pressure and room temperature, wherein the polymers demonstrate better efficiency than a homogeneous salen-cobalt catalyst. By combining the functions of gas storage and catalysts, this strategy provides a direction for cost-effective CO2 reduction processes.
Language英语
Funding Organization1,1 ; 1,1 ; 1,1 ; 1,1
URL查看原文
WOS IDWOS:000323624100028
Citation statistics
Cited Times:372[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/119092
Collection中国科学院大连化学物理研究所
Corresponding AuthorDeng WQ(邓伟侨)
Affiliation1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian Natl Lab Clean Energy, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China
2.China Three Gorges Univ, Coll Chem & Life Sci, Hubei Key Lab Nat Prod Res & Dev, Yichang 443002, Peoples R China
Recommended Citation
GB/T 7714
Xie, Yong,Wang, Ting-Ting,Liu, Xiao-Huan,et al. Capture and conversion of CO2 at ambient conditions by a conjugated microporous polymer[J]. NATURE COMMUNICATIONS,2013,4:1960.
APA Xie, Yong,Wang, Ting-Ting,Liu, Xiao-Huan,Zou, Kun,Deng, Wei-Qiao,&邓伟侨.(2013).Capture and conversion of CO2 at ambient conditions by a conjugated microporous polymer.NATURE COMMUNICATIONS,4,1960.
MLA Xie, Yong,et al."Capture and conversion of CO2 at ambient conditions by a conjugated microporous polymer".NATURE COMMUNICATIONS 4(2013):1960.
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