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学科主题物理化学
Capture and conversion of CO2 at ambient conditions by a conjugated microporous polymer
Xie, Yong1,2; Wang, Ting-Ting1; Liu, Xiao-Huan1; Zou, Kun2; Deng, Wei-Qiao1; Deng WQ(邓伟侨)
刊名NATURE COMMUNICATIONS
2013-06-01
ISSN2041-1723
DOI10.1038/ncomms2960
4页:1960
收录类别SCI
合作性质
文章类型Article
部门归属11
项目归属11T4
产权排名待补充
WOS标题词Science & Technology
资助者1,1 ; 1,1 ; 1,1 ; 1,1
类目[WOS]Multidisciplinary Sciences
研究领域[WOS]Science & Technology - Other Topics
关键词[WOS]METAL-ORGANIC FRAMEWORKS ; CARBON-DIOXIDE ; SURFACE-AREA ; CYCLIC CARBONATES ; HYDROGEN STORAGE ; CATALYSTS ; COMPLEXES ; EPOXIDES ; COPOLYMERIZATION ; NETWORKS
英文摘要Conjugated microporous polymers are a new class of porous materials with an extended pi-conjugation in an amorphous organic framework. Owing to the wide-ranging flexibility in the choice and design of components and the available control of pore parameters, these polymers can be tailored for use in various applications, such as gas storage, electronics and catalysis. Here we report a class of cobalt/aluminium-coordinated conjugated microporous polymers that exhibit outstanding CO2 capture and conversion performance at atmospheric pressure and room temperature. These polymers can store CO2 with adsorption capacities comparable to metal-organic frameworks. The cobalt-coordinated conjugated microporous polymers can also simultaneously function as heterogeneous catalysts for the reaction of CO2 and propylene oxide at atmospheric pressure and room temperature, wherein the polymers demonstrate better efficiency than a homogeneous salen-cobalt catalyst. By combining the functions of gas storage and catalysts, this strategy provides a direction for cost-effective CO2 reduction processes.
语种英语
资助者1,1 ; 1,1 ; 1,1 ; 1,1
原文出处查看原文
WOS记录号WOS:000323624100028
引用统计
被引频次:312[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/119092
专题中国科学院大连化学物理研究所
通讯作者Deng WQ(邓伟侨)
作者单位1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian Natl Lab Clean Energy, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China
2.China Three Gorges Univ, Coll Chem & Life Sci, Hubei Key Lab Nat Prod Res & Dev, Yichang 443002, Peoples R China
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GB/T 7714
Xie, Yong,Wang, Ting-Ting,Liu, Xiao-Huan,et al. Capture and conversion of CO2 at ambient conditions by a conjugated microporous polymer[J]. NATURE COMMUNICATIONS,2013,4:1960.
APA Xie, Yong,Wang, Ting-Ting,Liu, Xiao-Huan,Zou, Kun,Deng, Wei-Qiao,&邓伟侨.(2013).Capture and conversion of CO2 at ambient conditions by a conjugated microporous polymer.NATURE COMMUNICATIONS,4,1960.
MLA Xie, Yong,et al."Capture and conversion of CO2 at ambient conditions by a conjugated microporous polymer".NATURE COMMUNICATIONS 4(2013):1960.
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