DICP OpenIR
学科主题物理化学
Hybrid Artificial Photosynthetic Systems Comprising Semiconductors as Light Harvesters and Biomimetic Complexes as Molecular Cocatalysts
Wen, Fuyu; Li, Can1,2; Li C(李灿)
刊名ACCOUNTS OF CHEMICAL RESEARCH
2013-11-19
DOI10.1021/ar300224u
46期:11页:2355-2364
收录类别SCI
合作性质
文章类型Review
部门归属5
项目归属503
产权排名待补充
WOS标题词Science & Technology ; Physical Sciences
资助者1,1 ; 1,1 ; 1,1 ; 1,1
类目[WOS]Chemistry, Multidisciplinary
研究领域[WOS]Chemistry
关键词[WOS]HYDROGENASE ACTIVE-SITE ; PHOTOCATALYTIC H-2 EVOLUTION ; HIGH QUANTUM EFFICIENCY ; VISIBLE-LIGHT ; IRON HYDROGENASE ; CARBON-DIOXIDE ; WATER-OXIDATION ; CO2 REDUCTION ; ELECTROCATALYTIC REDUCTION ; CHARGE SEPARATION
英文摘要Solar fuel production through artificial photosynthesis may be a key to generating abundant and clean energy, thus addressing the high energy needs of the world's expanding population. As the crucial components of photosynthesis, the artificial photosynthetic system should be composed of a light harvester (e.g., semiconductor or molecular dye), a reduction cocatalyst (e.g., hydrogenase mimic, noble metal), and an oxidation cocatalyst (e.g., photosystem II mimic for oxygen evolution from water oxidation). Solar fuel production catalyzed by an artificial photosynthetic system starts from the absorption of sunlight by the light harvester, where charge separation takes place, followed by a charge transfer to the reduction and oxidation cocatalysts, where redox reaction processes occur. One of the most challenging problems is to develop an artificial photosynthetic solar fuel production system that is both highly efficient and stable. The assembly of cocatalysts on the semiconductor (light harvester) not only can facilitate the charge separation, but also can lower the activation energy or overpotential for the reactions. An efficient light harvester loaded with suitable reduction and oxidation cocatalysts is the key for high efficiency of artificial photosynthetic systems.
语种英语
资助者1,1 ; 1,1 ; 1,1 ; 1,1
原文出处查看原文
WOS记录号WOS:000327360800002
引用统计
被引频次:165[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/119179
专题中国科学院大连化学物理研究所
通讯作者Li C(李灿)
作者单位1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China
2.Dalian Natl Lab Clean Energy, Dalian 116023, Peoples R China
推荐引用方式
GB/T 7714
Wen, Fuyu,Li, Can,Li C. Hybrid Artificial Photosynthetic Systems Comprising Semiconductors as Light Harvesters and Biomimetic Complexes as Molecular Cocatalysts[J]. ACCOUNTS OF CHEMICAL RESEARCH,2013,46(11):2355-2364.
APA Wen, Fuyu,Li, Can,&李灿.(2013).Hybrid Artificial Photosynthetic Systems Comprising Semiconductors as Light Harvesters and Biomimetic Complexes as Molecular Cocatalysts.ACCOUNTS OF CHEMICAL RESEARCH,46(11),2355-2364.
MLA Wen, Fuyu,et al."Hybrid Artificial Photosynthetic Systems Comprising Semiconductors as Light Harvesters and Biomimetic Complexes as Molecular Cocatalysts".ACCOUNTS OF CHEMICAL RESEARCH 46.11(2013):2355-2364.
条目包含的文件
文件名称/大小 文献类型 版本类型 开放类型 使用许可
2013abg2s99piy.PDF(2360KB) 开放获取CC BY-NC-SA请求全文
个性服务
推荐该条目
保存到收藏夹
查看访问统计
导出为Endnote文件
谷歌学术
谷歌学术中相似的文章
[Wen, Fuyu]的文章
[Li, Can]的文章
[李灿]的文章
百度学术
百度学术中相似的文章
[Wen, Fuyu]的文章
[Li, Can]的文章
[李灿]的文章
必应学术
必应学术中相似的文章
[Wen, Fuyu]的文章
[Li, Can]的文章
[李灿]的文章
相关权益政策
暂无数据
收藏/分享
所有评论 (0)
暂无评论
 

除非特别说明,本系统中所有内容都受版权保护,并保留所有权利。