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学科主题: 物理化学
题名: Sulfonated carbon catalyzed oxidation of aldehydes to carboxylic acids by hydrogen peroxide
作者: Zhou, Lipeng1;  Dong, Beibei1;  Tang, Si1;  Ma, Hong1;  Chen, Chen2;  Yang, Xiaomei1;  Xu, Jie2
通讯作者: 杨晓梅
关键词: aldehyde ;  carboxylic acid ;  oxidation ;  hydrogen peroxide ;  sulfonated carbon
刊名: JOURNAL OF ENERGY CHEMISTRY
发表日期: 2013-07-01
卷: 22, 期:4, 页:659-664
收录类别: SCI
合作性质: 
文章类型: Article
部门归属: DNL06
项目归属: DNL0601
产权排名: 待补充
WOS标题词: Science & Technology ;  Physical Sciences ;  Technology
类目[WOS]: Chemistry, Applied ;  Chemistry, Physical ;  Energy & Fuels ;  Engineering, Chemical
资助者: 2,5
研究领域[WOS]: Chemistry ;  Energy & Fuels ;  Engineering
英文摘要: Sulfonated carbon as a strong and stable solid acid catalyst exhibited excellent catalytic performance in various acid-catalyzed reactions. Here, sulfonated carbon, as catalyst for oxidation reaction, was prepared via the carbonization of starch followed by sulfonation with concentrated sulfuric acid. N-2 physisorption, X-ray diffraction, Fourier transform infrared spectroscopy, X-ray fluorescence and acid-base titration were used to characterize the obtained materials. The catalytic activity of sulfonated carbon was studied in the oxidation of aldehydes to carboxylic acids using 30 wt% H2O2 as oxidant. This oxidation protocol works well for various aldehydes including aromatic and aliphatic aldehydes. The sulfonated carbon can be recycled for three times without obvious loss of activity.
关键词[WOS]: ORDERED MESOPOROUS CARBON ;  AROMATIC-ALDEHYDES ;  ORGANIC-COMPOUNDS ;  FUEL-CELLS ;  NANOTUBES
语种: 英语
原文出处: 查看原文
WOS记录号: WOS:000323239700017
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/119375
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Zhengzhou Univ, Coll Chem & Mol Engn, Zhengzhou 450001, Henan, Peoples R China
2.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian Natl Lab Clean Energy, State Key Lab Catalysis, Dalian 116023, Liaoning, Peoples R China

Recommended Citation:
Zhou, Lipeng,Dong, Beibei,Tang, Si,et al. Sulfonated carbon catalyzed oxidation of aldehydes to carboxylic acids by hydrogen peroxide[J]. JOURNAL OF ENERGY CHEMISTRY,2013,22(4):659-664.
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