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学科主题物理化学
Synthesis of functionalized 2-pyridones via Michael addition and cyclization reaction of amines, alkynes and dialkyl acetylene dicarboxylates
Chong, Qinglei; Xin, Xiaoyi; Wang, Chunxiang; Wu, Fan; Wan, Boshun; Wan BS(万伯顺)
刊名RSC ADVANCES
2013
DOI10.1039/c3ra43189d
3期:44页:21222-21226
收录类别SCI
合作性质
文章类型Article
部门归属2
项目归属202
产权排名待补充
WOS标题词Science & Technology ; Physical Sciences
资助者1,1 ; 1,1 ; 1,1 ; 1,1
类目[WOS]Chemistry, Multidisciplinary
研究领域[WOS]Chemistry
关键词[WOS]RING-FUSED 2-PYRIDONES ; REGIOSELECTIVE SYNTHESIS ; PYRIDONE ALKALOIDS ; DERIVATIVES ; MECHANISM ; TRANSFORMATIONS ; CYCLOADDITION ; HYDROLYSIS ; SCAFFOLDS ; MIGRATION
英文摘要The Michael addition and three-component cyclization reaction of amines, alkynes and dialkyl acetylene dicarboxylates to form pyridones has been developed. Aliphatic amines and aromatic amines could selectively be converted into N-alkyl-disubstituted 2-pyridones and N-aryl-trisubstituted 2-pyridones with good yields in the presence of wet ethanol, which means a suitable amount of water is required for this reaction. The Michael addition and cyclization reaction process was confirmed through deuterium-labeling experiments, intermediates isolation and control experiments.
语种英语
资助者1,1 ; 1,1 ; 1,1 ; 1,1
原文出处查看原文
WOS记录号WOS:000326056600005
引用统计
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/119481
专题中国科学院大连化学物理研究所
通讯作者Wan BS(万伯顺)
作者单位Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China
推荐引用方式
GB/T 7714
Chong, Qinglei,Xin, Xiaoyi,Wang, Chunxiang,et al. Synthesis of functionalized 2-pyridones via Michael addition and cyclization reaction of amines, alkynes and dialkyl acetylene dicarboxylates[J]. RSC ADVANCES,2013,3(44):21222-21226.
APA Chong, Qinglei,Xin, Xiaoyi,Wang, Chunxiang,Wu, Fan,Wan, Boshun,&万伯顺.(2013).Synthesis of functionalized 2-pyridones via Michael addition and cyclization reaction of amines, alkynes and dialkyl acetylene dicarboxylates.RSC ADVANCES,3(44),21222-21226.
MLA Chong, Qinglei,et al."Synthesis of functionalized 2-pyridones via Michael addition and cyclization reaction of amines, alkynes and dialkyl acetylene dicarboxylates".RSC ADVANCES 3.44(2013):21222-21226.
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