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学科主题物理化学
One-Pot Conversion of Cellulose to Ethylene Glycol with Multifunctional Tungsten-Based Catalysts
Wang, Aiqin; Zhang, Tao; Zhang T(张涛)
刊名ACCOUNTS OF CHEMICAL RESEARCH
2013-07-16
ISSN0001-4842
DOI10.1021/ar3002156
46期:7页:1377-1386
收录类别SCI
合作性质
文章类型Review
部门归属15
项目归属1501
产权排名待补充
WOS标题词Science & Technology ; Physical Sciences
资助者1,1 ; 1,1 ; 1,1 ; 1,1
类目[WOS]Chemistry, Multidisciplinary
研究领域[WOS]Chemistry
关键词[WOS]SUPPORTED RUTHENIUM CATALYSTS ; PHASE-TRANSFER CATALYSIS ; CARBIDE CATALYSTS ; SUPERCRITICAL WATER ; 1,2-PROPYLENE GLYCOL ; BIMETALLIC CATALYSTS ; SELECTIVE CONVERSION ; SUGAR ALCOHOLS ; CORN STALK ; HYDROLYSIS
英文摘要With diminishing fossil resources and increasing concerns about environmental issues, searching for alternative fuels has gained interest in recent years. Cellulose, as the most abundant nonfood biomass on earth, is a promising renewable feedstock for production of fuels and chemicals. In principle, the ample hydroxyl groups in the structure of cellulose make it an ideal feedstock for the production of industrially important polyols such as ethylene glycol (EG), according to the atom economy rule. However, effectively depolymerizing cellulose under mild conditions presents a challenge, due to the intra- and intermolecular hydrogen bonding network. In addition, control of product selectivity is complicated by the thermal instabilities of cellulose-derived sugars. A one-pot catalytic process that combines hydrolysis of cellulose and hydrogenation/hydrogenolysis of cellulose-derived sugars proves to be an efficient way toward the selective production of polyols from cellulose.
语种英语
资助者1,1 ; 1,1 ; 1,1 ; 1,1
原文出处查看原文
WOS记录号WOS:000322086600002
引用统计
被引频次:191[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/119601
专题中国科学院大连化学物理研究所
通讯作者Zhang T(张涛)
作者单位Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China
推荐引用方式
GB/T 7714
Wang, Aiqin,Zhang, Tao,Zhang T. One-Pot Conversion of Cellulose to Ethylene Glycol with Multifunctional Tungsten-Based Catalysts[J]. ACCOUNTS OF CHEMICAL RESEARCH,2013,46(7):1377-1386.
APA Wang, Aiqin,Zhang, Tao,&张涛.(2013).One-Pot Conversion of Cellulose to Ethylene Glycol with Multifunctional Tungsten-Based Catalysts.ACCOUNTS OF CHEMICAL RESEARCH,46(7),1377-1386.
MLA Wang, Aiqin,et al."One-Pot Conversion of Cellulose to Ethylene Glycol with Multifunctional Tungsten-Based Catalysts".ACCOUNTS OF CHEMICAL RESEARCH 46.7(2013):1377-1386.
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