DICP OpenIR
Subject Area物理化学
Recent progress in methane dehydroaromatization: From laboratory curiosities to promising technology
Ma, Shuqi1,2; Guo, Xiaoguang1; Zhao, Lingxiao1; Scott, Susannah3,4; Bao, Xinhe1; Bao XH(包信和)
KeywordDirect Conversion Methane Methane Dehydroaromatization Mo-based Catalyst
Source PublicationJOURNAL OF ENERGY CHEMISTRY
2013
Volume22Issue:1Pages:1-20
Indexed BySCI
Cooperation Status
SubtypeReview
Department5
Funding Project502
Contribution Rank待补充
WOS HeadingsScience & Technology ; Physical Sciences ; Technology
Funding Organization1,1 ; 1,1 ; 1,1 ; 1,1
WOS SubjectChemistry, Applied ; Chemistry, Physical ; Energy & Fuels ; Engineering, Chemical
WOS Research AreaChemistry ; Energy & Fuels ; Engineering
WOS KeywordMO-BASED CATALYSTS ; HYDROTHERMAL POST-SYNTHESIS ; BRONSTED ACID SITES ; TEMPERATURE NONOXIDATIVE ACTIVATION ; GALLOALUMINOSILICATE MFI ZEOLITE ; IMPREGNATED HZSM-5 CATALYSTS ; HIGHLY STABLE PERFORMANCE ; SUPERSONIC JET EXPANSION ; SINGLE-PASS CONVERSION ; MO-95 NMR-SPECTROSCOPY
AbstractDirect conversion of methane to benzene or other valuable chemicals is a very promising process for the efficient application of natural gas. Compared with conversion processes that require oxidants, non-oxidative direct conversion is more attractive due to high selectivity to the target product. In this paper, an alternative route for methane dehydrogenation and selective conversion to benzene and hydrogen without the participation of oxygen is discussed. A brief review of the catalysts used in methane dehydroaromatization (MDA) is first given, followed by our current understanding of the location and the active phase of Mo species, the reaction mechanism, the mechanism of carbonaceous deposit and the deactivation of Mo/zeolite catalysts are systematically discussed. Ways to improve the catalytic activity and stability are described in detail based on catalyst and reaction as well as reactor design. Future prospects for methane dehydroaromatization process are also presented.
Language英语
Funding Organization1,1 ; 1,1 ; 1,1 ; 1,1
URL查看原文
WOS IDWOS:000318050700002
Citation statistics
Cited Times:84[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/119624
Collection中国科学院大连化学物理研究所
Corresponding AuthorBao XH(包信和)
Affiliation1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Liaoning, Peoples R China
2.Henan Polytech Univ, Sch Phys & Chem, Jiaozuo 454000, Henan, Peoples R China
3.Univ Calif Santa Barbara, Dept Chem & Biochem, Santa Barbara, CA 93106 USA
4.Univ Calif Santa Barbara, Dept Chem Engn, Santa Barbara, CA 93106 USA
Recommended Citation
GB/T 7714
Ma, Shuqi,Guo, Xiaoguang,Zhao, Lingxiao,et al. Recent progress in methane dehydroaromatization: From laboratory curiosities to promising technology[J]. JOURNAL OF ENERGY CHEMISTRY,2013,22(1):1-20.
APA Ma, Shuqi,Guo, Xiaoguang,Zhao, Lingxiao,Scott, Susannah,Bao, Xinhe,&包信和.(2013).Recent progress in methane dehydroaromatization: From laboratory curiosities to promising technology.JOURNAL OF ENERGY CHEMISTRY,22(1),1-20.
MLA Ma, Shuqi,et al."Recent progress in methane dehydroaromatization: From laboratory curiosities to promising technology".JOURNAL OF ENERGY CHEMISTRY 22.1(2013):1-20.
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