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学科主题: 物理化学
题名: Synthesis of gasoline from syngas in a dual layer catalyst system
作者: Wang, Chun1, 3;  Zhang, Dazhi2;  Fang, Chuanyan1;  Ge, Qingjie1;  Xu, Hengyong1
通讯作者: 葛庆杰 ;  徐恒泳
关键词: Gasoline range hydrocarbons ;  Syngas ;  Catalyst arrangement ;  Pd ;  HZSM-5
刊名: FUEL
发表日期: 2014-10-15
DOI: 10.1016/j.fuel.2014.05.045
卷: 134, 页:11-16
收录类别: SCI
合作性质: 
文章类型: Article
部门归属: DNL19
项目归属: DNL1902
产权排名: 待补充
WOS标题词: Science & Technology ;  Technology
类目[WOS]: Energy & Fuels ;  Engineering, Chemical
资助者: 1,1
研究领域[WOS]: Energy & Fuels ;  Engineering
英文摘要: Catalytic reaction of syngas to gasoline range hydrocarbons was investigated over a hybrid catalyst, which is composed of a DME synthesis catalyst (CZAA) and a Pd modified HZSM-5 (PdZSM-5). The results showed that the existence of inert layer in CZAA/PdZSM-5 was beneficial to the formation of C-5-C-11 hydrocarbons. A 62% of CO conversion and a 66% of gasoline content in hydrocarbon products could be obtained over a dual layer catalyst system. In addition, the results indicated that the product hydrocarbon distribution was mainly determined by PdZSM-5, and the modification of Pd on HZSM-5 favors the formation of isoparaffin products at operated conditions. (C) 2014 Elsevier Ltd. All rights reserved.
关键词[WOS]: FISCHER-TROPSCH SYNTHESIS ;  PRODUCT SELECTIVITY ;  LIQUID HYDROCARBONS ;  SYNTHESIS GAS ;  CONVERSION ;  METHANOL ;  ZSM-5 ;  HYDROISOMERIZATION ;  TRANSFORMATION ;  SIZE
语种: 英语
原文出处: 查看原文
WOS记录号: WOS:000340304100002
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/119731
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian Natl Lab Clean Energy DNL, Dalian 116023, Peoples R China
2.BP Dalian Energy Innovat Lab, Dalian 116023, Peoples R China
3.Univ Chinese Acad Sci, Beijing 100039, Peoples R China

Recommended Citation:
Wang, Chun,Zhang, Dazhi,Fang, Chuanyan,et al. Synthesis of gasoline from syngas in a dual layer catalyst system[J]. FUEL,2014,134:11-16.
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