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学科主题: 物理化学
题名: Slice imaging of methyl bromide photofragmentation at 193 nm
作者: Wang, Fengyan1, 2;  Lipciuc, M. Laura1;  Kartakoullis, Andreas1, 4;  Glodic, Pavle1, 4;  Samartzis, Peter C.1;  Yang, Xueming3;  Kitsopoulos, Theofanis N.1, 4
通讯作者: Theofanis N. Kitsopoulos
刊名: PHYSICAL CHEMISTRY CHEMICAL PHYSICS
发表日期: 2014
DOI: 10.1039/c3cp53139b
卷: 16, 期:2, 页:599-606
收录类别: SCI
合作性质: 
文章类型: Article
部门归属: 11
项目归属: 1102
产权排名: 待补充
WOS标题词: Science & Technology ;  Physical Sciences
类目[WOS]: Chemistry, Physical ;  Physics, Atomic, Molecular & Chemical
资助者: 3,6
研究领域[WOS]: Chemistry ;  Physics
英文摘要: The photodissociation of methyl bromide at 193 nm is studied using slice imaging. From the measured photofragment translational energy and angular distributions we were able to extract methyl-state-specific dissociation channel yields and crossing probabilities between (3)Q(0) and (1)Q(1) surfaces. The angular distributions for the Bromine photofragments show a strong dependence on the total translational energy release. Nonadiabatic transition probabilities from the (3)Q(0) to (1)Q(1) surface dominate the dynamics in this excitation energy region and for most of the methyl vibrational states probed.
关键词[WOS]: MULTIPHOTON IONIZATION SPECTROSCOPY ;  A-BAND ;  PHOTODISSOCIATION ;  ALIGNMENT ;  CH3BR ;  EXCITATION ;  MOLECULES ;  DYNAMICS ;  ROTATION ;  INITIO
语种: 英语
原文出处: 查看原文
WOS记录号: WOS:000327888100025
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/119759
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Fdn Res & Technol Hellas, Inst Elect Struct & Laser, Iraklion 71110, Greece
2.Fudan Univ, Dept Chem, Shanghai 200433, Peoples R China
3.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China
4.Univ Crete, Dept Chem, Iraklion 71003, Greece

Recommended Citation:
Wang, Fengyan,Lipciuc, M. Laura,Kartakoullis, Andreas,et al. Slice imaging of methyl bromide photofragmentation at 193 nm[J]. PHYSICAL CHEMISTRY CHEMICAL PHYSICS,2014,16(2):599-606.
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