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题名: Synthesis of SAPO-35 molecular sieve and its catalytic properties in the methanol-to-olefins reaction
作者: Li Bing1;  Tian Peng1;  Li Jinzhe1;  Chen Jingrun1, 2;  Yuan Yangyang1, 2;  Su Xiong1, 2;  Fan Dong1, 2;  Wei Yingxu1;  Qi Yue1;  Liu Zhongmin1
关键词: SAPO-35 ;  Methanol to olefins ;  SAPO-34 ;  Coke species ;  Deactivation
刊名: CHINESE JOURNAL OF CATALYSIS
发表日期: 2013-04-01
DOI: 10.1016/S1872-2067(12)60557-9
卷: 34, 期:4, 页:798-807
收录类别: SCI
文章类型: Article
WOS标题词: Science & Technology ;  Physical Sciences ;  Technology
类目[WOS]: Chemistry, Applied ;  Chemistry, Physical ;  Engineering, Chemical
研究领域[WOS]: Chemistry ;  Engineering
英文摘要: SAPO-35 molecular sieve samples with different Si contents were hydrothermally synthesized using hexamethyleneimine as the template and characterized by XRD, XRF, SEM, MAS NMR, XPS and N-2 physisorption. Three SAPO-35 samples were tested as methanol-to-olefins catalysts. After the reaction, the evolution of coke species was investigated over SAPO-35 and SAPO-34 catalysts with similar Si concentrations. A correlation between the cage size of the molecular sieves and the coke species was obtained. (C) 2013, Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by Elsevier RV. All rights reserved.
关键词[WOS]: HYDROCARBONS REACTION ;  SHAPE-SELECTIVITY ;  CONVERSION ;  DEACTIVATION ;  CAVITIES
语种: 英语
WOS记录号: WOS:000318750500022
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/137472
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Chinese Acad Sci, Dalian Inst Chem Phys, Natl Engn Lab Methanol To Olefins, Dalian Natl Lab Clean Energy, Dalian 116023, Liaoning, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China

Recommended Citation:
Li Bing,Tian Peng,Li Jinzhe,et al. Synthesis of SAPO-35 molecular sieve and its catalytic properties in the methanol-to-olefins reaction[J]. CHINESE JOURNAL OF CATALYSIS,2013,34(4):798-807.
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