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Rh(III)-catalyzed oxidative synthesis of pyrazoles from azomethines and acrylamides
Zhen Wencui1,2; Du Zhengyin1; Li Xingwei2
关键词Rhodium(Iii) C-h Bond Activation Acrylamide Azomethine C-n Coupling Pyrazole
刊名CHINESE JOURNAL OF CATALYSIS
2013-04-01
DOI10.1016/S1872-2067(12)60584-1
34期:4页:679-683
收录类别SCI
文章类型Article
WOS标题词Science & Technology ; Physical Sciences ; Technology
类目[WOS]Chemistry, Applied ; Chemistry, Physical ; Engineering, Chemical
研究领域[WOS]Chemistry ; Engineering
关键词[WOS]H BOND-CLEAVAGE ; N-HETEROCYCLIC CARBENES ; C-H ; INTERNAL ALKYNES ; CATALYZED HYDROFORMYLATION ; RHODIUM CATALYSIS ; BENZOIC-ACIDS ; ACTIVATION ; COUPLING/CYCLIZATION ; BENZAMIDES
英文摘要A cationic Rh(III) complex has been developed to catalyze the oxidative coupling of azomethine imines to acrylamides, to give trisubstituted pyrazoles in moderate yield. In this process, the olefinic C-H bond of the acrylamide undergoes C-H activation, and the reaction subsequently proceeds via a different selectivity to that reported for the coupling of acrylate esters. (C) 2013, Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by Elsevier B.V. All rights reserved.
语种英语
WOS记录号WOS:000318750500007
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被引频次:6[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/137521
专题中国科学院大连化学物理研究所
作者单位1.Northwest Normal Univ, Coll Chem & Chem Engn, Key Lab Ecoenvironm Related Polymer Mat, Minist Educ,Gansu Key Lab Polymer Mat, Lanzhou 730070, Gansu, Peoples R China
2.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Liaoning, Peoples R China
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Zhen Wencui,Du Zhengyin,Li Xingwei. Rh(III)-catalyzed oxidative synthesis of pyrazoles from azomethines and acrylamides[J]. CHINESE JOURNAL OF CATALYSIS,2013,34(4):679-683.
APA Zhen Wencui,Du Zhengyin,&Li Xingwei.(2013).Rh(III)-catalyzed oxidative synthesis of pyrazoles from azomethines and acrylamides.CHINESE JOURNAL OF CATALYSIS,34(4),679-683.
MLA Zhen Wencui,et al."Rh(III)-catalyzed oxidative synthesis of pyrazoles from azomethines and acrylamides".CHINESE JOURNAL OF CATALYSIS 34.4(2013):679-683.
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