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A robust Ru-PNNP catalyst system for the asymmetric hydrogenation of alpha,beta-unsaturated ketones to allylic alcohol
Lu, Sheng-Mei1,2; Gao, Qiang1; Li, Jun1; Liu, Yan1; Li, Can1
关键词Ruthenium Biphosphinobioxazoline Hydrogenation Unsaturated Ketones Allylic Alcohol
刊名TETRAHEDRON LETTERS
2013-12-18
DOI10.1016/j.tetlet.2013.10.051
54期:51页:7013-7016
收录类别SCI ; IC ; CCR
文章类型Article
WOS标题词Science & Technology ; Physical Sciences
类目[WOS]Chemistry, Organic
研究领域[WOS]Chemistry
关键词[WOS]HIGHLY ENANTIOSELECTIVE HYDROGENATION ; STEREOSELECTIVE HYDROGENATION ; HETEROAROMATIC-COMPOUNDS ; RUTHENIUM(II) COMPLEX ; AROMATIC KETONES ; CHIRAL LIGAND ; HYDROSILYLATION ; EFFICIENT ; ALPHA
英文摘要A robust and stable Ru-Biphosphinobioxazoline catalyst system is discovered for the highly enantioselective hydrogenation of enones to allylic alcohols. A series of acyclic alpha,beta-unsaturated ketones react well affording the desired products in high yields (up to 98%) and enantioselectivities (up to 98% ee). Simple manipulation process and tolerance of water and air make this catalysis more practical and appealing. (C) 2013 Elsevier Ltd. All rights reserved.
语种英语
WOS记录号WOS:000327577200008
引用统计
被引频次:6[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/137645
专题中国科学院大连化学物理研究所
作者单位1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China
2.Cent China Normal Univ, Coll Chem, Minist Educ, Key Lab Pesticide & Chem Biol, Wuhan 430079, Hubei, Peoples R China
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GB/T 7714
Lu, Sheng-Mei,Gao, Qiang,Li, Jun,et al. A robust Ru-PNNP catalyst system for the asymmetric hydrogenation of alpha,beta-unsaturated ketones to allylic alcohol[J]. TETRAHEDRON LETTERS,2013,54(51):7013-7016.
APA Lu, Sheng-Mei,Gao, Qiang,Li, Jun,Liu, Yan,&Li, Can.(2013).A robust Ru-PNNP catalyst system for the asymmetric hydrogenation of alpha,beta-unsaturated ketones to allylic alcohol.TETRAHEDRON LETTERS,54(51),7013-7016.
MLA Lu, Sheng-Mei,et al."A robust Ru-PNNP catalyst system for the asymmetric hydrogenation of alpha,beta-unsaturated ketones to allylic alcohol".TETRAHEDRON LETTERS 54.51(2013):7013-7016.
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