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Exceptional activity for direct synthesis of phenol from benzene over PMoV@MOF with O-2
Yang, Hua1,2; Li, Jun1,2; Wang, Lianyue1,2; Dai, Wen1,2,3; Lv, Ying1,2; Gao, Shuang1,2
关键词Polyoxometalates Mofs Oxygen Benzene Phenol
刊名CATALYSIS COMMUNICATIONS
2013-05-05
DOI10.1016/j.catcom.2013.02.013
35页:101-104
收录类别SCI
文章类型Article
WOS标题词Science & Technology ; Physical Sciences
类目[WOS]Chemistry, Physical
研究领域[WOS]Chemistry
关键词[WOS]METAL-ORGANIC FRAMEWORK ; SELECTIVE HYDROXYLATION ; MESOPOROUS SILICA ; OXIDATION ; CATALYSTS ; OXIDE ; REACTIVITY ; STABILITY ; DIOXYGEN ; HYDROGEN
英文摘要Three novel catalysts named as PMo12-nVn@HKUST-1 (n=1-3) were designed and obtained through encapsulating vanadium-doped Keggin polyoxometalates (POMs) PMo12-n V-n into the framework HKUST-1 (also denoted as Cu-3(BTC)(2), MOF-199). The character structure of PMo12-n V-n@HKUST-1 was elucidated through the single crystal XRD of PMo11V@HKUST-1. Reaction rate could be greatly enhanced by PMo12-n V-n@HKUST-1 in liquid hydroxylation of benzene with O-2. Only in 20 min, a high TOF (442 h(-1)) of PMo9V3@HKUST-1 was obtained. (C) 2013 Elsevier B.V. All rights reserved.
语种英语
WOS记录号WOS:000317883100020
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被引频次:28[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/137675
专题中国科学院大连化学物理研究所
作者单位1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China
2.Dalian Natl Lab Clean Energy, Dalian 116023, Peoples R China
3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
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Yang, Hua,Li, Jun,Wang, Lianyue,et al. Exceptional activity for direct synthesis of phenol from benzene over PMoV@MOF with O-2[J]. CATALYSIS COMMUNICATIONS,2013,35:101-104.
APA Yang, Hua,Li, Jun,Wang, Lianyue,Dai, Wen,Lv, Ying,&Gao, Shuang.(2013).Exceptional activity for direct synthesis of phenol from benzene over PMoV@MOF with O-2.CATALYSIS COMMUNICATIONS,35,101-104.
MLA Yang, Hua,et al."Exceptional activity for direct synthesis of phenol from benzene over PMoV@MOF with O-2".CATALYSIS COMMUNICATIONS 35(2013):101-104.
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