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题名: Improved dehydrogenation/rehydrogenation performance of LiBH4 by doping mesoporous Fe2O3 or/and TiF3
作者: Zhang, Hui1, 2;  Cao, Zhong1;  Sun, Li-Xian2, 3;  Sun, Yu-Jia4;  Xu, Fen5;  Liu, Hui1, 2;  Zhang, Jian2;  Huang, Zi-Qiang2;  Jiang, Xia2;  Li, Zhi-Bao2;  Liu, Shuang2;  Wang, Shuang2;  Jiao, Cheng-Li2;  Zhou, Huai-Ying3;  Sawada, Yutaka6
关键词: LiBH4 ;  Mesoporous iron oxide ;  Trifluoride antimony ;  Co-doped system ;  Hydrogen storage
刊名: JOURNAL OF THERMAL ANALYSIS AND CALORIMETRY
发表日期: 2013-06-01
DOI: 10.1007/s10973-012-2721-8
卷: 112, 期:3, 页:1407-1414
收录类别: SCI
文章类型: Article
WOS标题词: Science & Technology ;  Physical Sciences
类目[WOS]: Chemistry, Analytical ;  Chemistry, Physical
研究领域[WOS]: Chemistry
英文摘要: The LiBH4 + mesoporous Fe2O3 (defined as M-Fe2O3) mono-doped and LiBH4 + M-Fe2O3 + TiF3 co-doped hybrid materials were prepared by ball milling process. A variety of characterization methods, such as thermogravimetric, differential scanning calorimetry, X-ray diffraction, and pressure-composition-temperature instrument, were used for examinations of the two materials' performances of storage/release of hydrogen, catalytic activity, kinetics, and thermodynamics. All the results showed that the M-Fe2O3 prepared in laboratory exhibited a good catalytic effect. Compared with the performance of M-Fe2O3 mono-doped system, M-Fe2O3 and TiF3 co-doped mode exhibits a better performance using the same additive content. Thus, the M-Fe2O3 and TiF3 co-doped mode possesses a collaborative catalytic utility with the LiBH4 hydrogen performance improved, showing a promising application.
关键词[WOS]: HYDROGEN STORAGE PROPERTIES ;  METAL-HYDRIDES ;  LITHIUM BOROHYDRIDE ;  CARBON ;  NAALH4 ;  DECOMPOSITION ;  NANOPARTICLES ;  DESORPTION ;  AMMONIA ;  SYSTEM
语种: 英语
WOS记录号: WOS:000319358500031
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/137691
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Changsha Univ Sci & Technol, Sch Chem & Biol Engn, Hunan Prov Key Lab Mat Protect Elect Power & Tran, Changsha 410004, Hunan, Peoples R China
2.Chinese Acad Sci, Dalian Inst Chem Phys, Mat & Thermochem Lab, Dalian 116023, Peoples R China
3.Guilin Univ Elect Technol, Fac Mat Sci & Engn, Guilin 541004, Peoples R China
4.Wuhan Univ, Coll Chem & Mol Sci, Wuhan 430072, Peoples R China
5.Guilin Univ Elect Technol, Dept Mat Sci & Engn, Guilin 541004, Peoples R China
6.Tokyo Polytech Univ, Grad Sch Engn, Ctr Hyper Media Res, Atsugi, Kanagawa 2430297, Japan

Recommended Citation:
Zhang, Hui,Cao, Zhong,Sun, Li-Xian,et al. Improved dehydrogenation/rehydrogenation performance of LiBH4 by doping mesoporous Fe2O3 or/and TiF3[J]. JOURNAL OF THERMAL ANALYSIS AND CALORIMETRY,2013,112(3):1407-1414.
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