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Efficient Coherent Population Transfer of D-2 Molecules by Stark-induced Adiabatic Raman Passage
Wang, Tao1; Yang, Tian-gang1,2; Xiao, Chun-lei1; Dai, Dong-xu1; Yang, Xue-ming1
关键词Stark-induced Adiabatic Raman Passage D-2 Vibrational Excitation Molecular Beam
刊名CHINESE JOURNAL OF CHEMICAL PHYSICS
2013-02-27
DOI10.1063/1674-0068/26/01/8-12
26期:1页:8-12
收录类别SCI
文章类型Article
WOS标题词Science & Technology ; Physical Sciences
类目[WOS]Physics, Atomic, Molecular & Chemical
研究领域[WOS]Physics
关键词[WOS]DIFFERENTIAL CROSS-SECTIONS ; STATE ; SPECTROSCOPY ; RESONANCES ; HD ; D2
英文摘要Preparation of a high flux of hydrogen molecules in a specific vibrationally excited state is the major prerequisite and challenge in scattering experiments that use vibrationally excited hydrogen molecules as the target. The widely used scheme of stimulated Raman pumping suffers from coherent population return which severely limits the excitation efficiency. Recently we successfully transferred D-2 molecules in the molecular beam from (v=0, J=0) to (v=1, J=0) level, with the scheme of Stark-induced adiabatic Raman passage. As high as 75% of the excitation efficiency was achieved. This excitation technique promise to be a unique tool for crossed beam and beam-surface scattering experiments which aim to reveal the role of vibrational excitation of hydrogen molecules in the chemical reaction.
语种英语
WOS记录号WOS:000316093500002
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被引频次:2[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/137916
专题中国科学院大连化学物理研究所
作者单位1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116024, Peoples R China
2.Dalian Univ Technol, Sch Phys & Optoelect Engn, Dalian 116024, Peoples R China
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GB/T 7714
Wang, Tao,Yang, Tian-gang,Xiao, Chun-lei,et al. Efficient Coherent Population Transfer of D-2 Molecules by Stark-induced Adiabatic Raman Passage[J]. CHINESE JOURNAL OF CHEMICAL PHYSICS,2013,26(1):8-12.
APA Wang, Tao,Yang, Tian-gang,Xiao, Chun-lei,Dai, Dong-xu,&Yang, Xue-ming.(2013).Efficient Coherent Population Transfer of D-2 Molecules by Stark-induced Adiabatic Raman Passage.CHINESE JOURNAL OF CHEMICAL PHYSICS,26(1),8-12.
MLA Wang, Tao,et al."Efficient Coherent Population Transfer of D-2 Molecules by Stark-induced Adiabatic Raman Passage".CHINESE JOURNAL OF CHEMICAL PHYSICS 26.1(2013):8-12.
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