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OH spillover from a gamma-Al2O3 support in the partial oxidation of methane over Ru/Al2O3
Wang, DZ; Li, ZL; Luo, CR; Weng, WZ; Wan, HL
关键词Kinetics Modelling Multiphase Reactions Selectivity Methane Oxidation Spillover
刊名CHEMICAL ENGINEERING SCIENCE
2003-02-01
DOI10.1016/S0009-2509(02)00620-6
58期:3-6页:887-893
收录类别ISTP ; SCI
文章类型Article
WOS标题词Science & Technology ; Technology
类目[WOS]Engineering, Chemical
研究领域[WOS]Engineering
关键词[WOS]SYNTHESIS GAS ; CATALYSTS ; TAP ; SYSTEM
英文摘要The microkinetics of the oxidation of methane on Ru/Al2O3 is developed using a TAP reactor. The shapes of the response curves of reactants and products are used to identify the elementary reactions and their rate parameters. The support, which strongly adsorbs H2O, participates in the reaction sequence through its supply of hydroxyl to metal particles by spillover, and this step is of kinetic significance. The relative rates of the elementary reactions that give overall partial oxidation or total oxidation are discussed. (C) 2003 Elsevier Science Ltd. All rights reserved.
语种英语
WOS记录号WOS:000181575600045
引用统计
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/138216
专题中国科学院大连化学物理研究所
作者单位1.Tsing Hua Univ, Dept Chem Engn, Beijing 100084, Peoples R China
2.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China
3.Xiamen Univ, Dept Chem, State Key Lab Phys Chem Solid Surfaces, Xiamen 361005, Peoples R China
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GB/T 7714
Wang, DZ,Li, ZL,Luo, CR,et al. OH spillover from a gamma-Al2O3 support in the partial oxidation of methane over Ru/Al2O3[J]. CHEMICAL ENGINEERING SCIENCE,2003,58(3-6):887-893.
APA Wang, DZ,Li, ZL,Luo, CR,Weng, WZ,&Wan, HL.(2003).OH spillover from a gamma-Al2O3 support in the partial oxidation of methane over Ru/Al2O3.CHEMICAL ENGINEERING SCIENCE,58(3-6),887-893.
MLA Wang, DZ,et al."OH spillover from a gamma-Al2O3 support in the partial oxidation of methane over Ru/Al2O3".CHEMICAL ENGINEERING SCIENCE 58.3-6(2003):887-893.
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