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Interference of quantized transition-state pathways in the H+D2 -> D+HD chemical reaction
Dai, DX; Wang, CC; Harich, SA; Wang, XY; Yang, XM; Chao, SD; Skodje, RT
刊名SCIENCE
2003-06-13
300期:5626页:1730-1734
收录类别SCI
文章类型Article
WOS标题词Science & Technology
类目[WOS]Multidisciplinary Sciences
研究领域[WOS]Science & Technology - Other Topics
关键词[WOS]DIFFERENTIAL CROSS-SECTIONS ; HYDROGEN-EXCHANGE REACTION ; SPECTRAL QUANTIZATION ; H+D-2->HD+D REACTION ; TRIPLET KETENE ; SCATTERING ; DYNAMICS ; RESONANCE ; THRESHOLDS ; H+D-2
英文摘要The collision-energy dependence of the state-resolved differential cross section at a specific backward-scattering angle for the reaction H + D-2 --> D + HD is measured with the D-atom Rydberg "tagging" time-of-flight technique. The reaction was modeled theoretically with converged quantum scattering calculations that provided physical interpretation of the observations. Oscillations in the differential cross sections in the backward-scattering direction are clearly observed and are attributed to the transition-state structures that originate from the interferences of different quantized transition-state pathways.
语种英语
WOS记录号WOS:000183459700046
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被引频次:101[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/138292
专题中国科学院大连化学物理研究所
作者单位1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian, Peoples R China
2.Acad Sinica, Inst Atom & Mol Sci, Taipei, Taiwan
3.Natl Taiwan Univ, Dept Chem, Taipei 10764, Taiwan
4.Natl Tsing Hua Univ, Dept Chem, Hsinchu, Taiwan
5.Univ Colorado, Dept Chem & Biochem, Boulder, CO 80309 USA
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GB/T 7714
Dai, DX,Wang, CC,Harich, SA,et al. Interference of quantized transition-state pathways in the H+D2 -> D+HD chemical reaction[J]. SCIENCE,2003,300(5626):1730-1734.
APA Dai, DX.,Wang, CC.,Harich, SA.,Wang, XY.,Yang, XM.,...&Skodje, RT.(2003).Interference of quantized transition-state pathways in the H+D2 -> D+HD chemical reaction.SCIENCE,300(5626),1730-1734.
MLA Dai, DX,et al."Interference of quantized transition-state pathways in the H+D2 -> D+HD chemical reaction".SCIENCE 300.5626(2003):1730-1734.
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