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题名: Time-dependent wave packet approach to Rabi oscillation in strong laser field
作者: Meng, QT;  Yang, GH;  Han, KL
关键词: Rabi oscillation ;  strong laser fields ;  multiphoton ionization ;  wave packet propagation ;  chemical reaction control
刊名: INTERNATIONAL JOURNAL OF QUANTUM CHEMISTRY
发表日期: 2003-10-05
DOI: 10.1002/qua.10712
卷: 95, 期:1, 页:30-36
收录类别: SCI
文章类型: Article
WOS标题词: Science & Technology ;  Physical Sciences
类目[WOS]: Chemistry, Physical ;  Mathematics, Interdisciplinary Applications ;  Physics, Atomic, Molecular & Chemical
研究领域[WOS]: Chemistry ;  Mathematics ;  Physics
英文摘要: The phenomenon of Rabi oscillation is obtained in the investigation of the NO multiphoton ionization (MPI) in femtosecond laser fields. The "split operator-Fourier transform" method of wave packet propagation is used in the representation of Rabi oscillation of population in each electronic state of NO molecule. The origin of Rabi oscillation and the effect on multiphoton ionization is analyzed. The high-frequency oscillation riding on the top of Rabi oscillation is attributed to the nonrotating wave component in strong laser fields. Also illustrated is that through adjusting the pump-probe delay time and the laser intensity appropriately the control of the ionization yield can be realized. This idea may be important for the laser control of chemical reaction. (C) 2003 Wiley Periodicals, Inc. Int J Quantum Chem 95: 30-36, 2003.
关键词[WOS]: MULTIPHOTON IONIZATION ;  SCHRODINGER-EQUATION ;  SPECTRAL METHOD ;  PULSES ;  PHOTOIONIZATION ;  POTENTIALS ;  FREQUENCY ;  MOLECULES ;  NA2
语种: 英语
WOS记录号: WOS:000185157200003
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/138386
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China

Recommended Citation:
Meng, QT,Yang, GH,Han, KL. Time-dependent wave packet approach to Rabi oscillation in strong laser field[J]. INTERNATIONAL JOURNAL OF QUANTUM CHEMISTRY,2003,95(1):30-36.
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