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Thermal evolution of the structure of a Mg-Al-CO3 layered double hydroxide: Sorption reversibility aspects
Kim, Y; Yang, WS; Liu, PKT; Sahimi, M; Tsotsis, TT
Source PublicationINDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
2004-08-04
DOI10.1021/ie0308036
Volume43Issue:16Pages:4559-4570
Indexed BySCI
SubtypeArticle
WOS HeadingsScience & Technology ; Technology
WOS SubjectEngineering, Chemical
WOS Research AreaEngineering
WOS KeywordHYDROTALCITE-LIKE COMPOUNDS ; X-RAY-DIFFRACTION ; COMPOUNDS HTLCS ; CO2 ADSORPTION ; MG ; CATALYSTS ; MG/AL ; TEMPERATURES ; CARBONATE ; OXIDATION
AbstractIn our prior study, we employed several in-situ techniques to investigate the thermal evolution of the structure of a Mg-Al-CO3 layered double hydroxide (LDH) under an inert atmosphere and proposed a model to describe the structural evolution of the Mg-Al-CO3 LDH structure. In this paper we present results of our ongoing investigations with these materials pertaining to their sorption characteristics and thermal reversibility under both inert and reactive atmospheres. The experimental observations are shown to be consistent with the structural model for the LDH previously proposed. The structure, sorption characteristics, and thermal reversibility of these materials are of importance in their use for the preparation of CO2-permselective membranes for high-temperature membrane reactor applications.
Language英语
WOS IDWOS:000222979900011
Citation statistics
Cited Times:27[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/138427
Collection中国科学院大连化学物理研究所
Affiliation1.Univ So Calif, Dept Chem Engn, Los Angeles, CA 90089 USA
2.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China
3.Media & Proc Technol Inc, Pittsburgh, PA 15238 USA
Recommended Citation
GB/T 7714
Kim, Y,Yang, WS,Liu, PKT,et al. Thermal evolution of the structure of a Mg-Al-CO3 layered double hydroxide: Sorption reversibility aspects[J]. INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,2004,43(16):4559-4570.
APA Kim, Y,Yang, WS,Liu, PKT,Sahimi, M,&Tsotsis, TT.(2004).Thermal evolution of the structure of a Mg-Al-CO3 layered double hydroxide: Sorption reversibility aspects.INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,43(16),4559-4570.
MLA Kim, Y,et al."Thermal evolution of the structure of a Mg-Al-CO3 layered double hydroxide: Sorption reversibility aspects".INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH 43.16(2004):4559-4570.
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