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题名: Femtosecond pump-probe photodissociation of OClO: direct observation of the (2)A(1) state and the role of accidental multiphoton resonance
作者: Sun, ZG;  Lou, NQ;  Nyman, G
刊名: CHEMICAL PHYSICS LETTERS
发表日期: 2004-07-21
DOI: 10.1016/j.cplett.2004.06.030
卷: 393, 期:1-3, 页:204-208
收录类别: SCI
文章类型: Article
WOS标题词: Science & Technology ;  Physical Sciences
类目[WOS]: Chemistry, Physical ;  Physics, Atomic, Molecular & Chemical
研究领域[WOS]: Chemistry ;  Physics
英文摘要: Previous pump-probe experiments on the OCIO molecule are analyzed and a consistent interpretation of the experimental observations is proposed. We demonstrate that a direct observation of the very weak (2)A(1) state of OCIO is possible with a proper femtosecond pulse, and suggest that it is necessary to introduce an accidental resonance of the probe pulse with the highly excited D or E states for understanding the observed distinct photodissociation dynamics of the (2)A(2) state using pump pulses of slightly different wavelengths. A transient abnormal peak, observed in the OCIO+ ion signal after a stronger excitation, is also convincingly interpreted. (C) 2004 Elsevier B.V. All rights reserved.
关键词[WOS]: WAVE-PACKET MOTION ;  CHLORINE DIOXIDE ;  IONIZATION PATH ;  SPECTROSCOPY ;  DYNAMICS ;  PHOTOABSORPTION ;  FRAGMENTATION ;  PERTURBATION ;  PHASE ;  PULSE
语种: 英语
WOS记录号: WOS:000222887700037
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/138430
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China
2.Univ Gothenburg, Dept Chem, SE-41296 Gothenburg, Sweden

Recommended Citation:
Sun, ZG,Lou, NQ,Nyman, G. Femtosecond pump-probe photodissociation of OClO: direct observation of the (2)A(1) state and the role of accidental multiphoton resonance[J]. CHEMICAL PHYSICS LETTERS,2004,393(1-3):204-208.
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