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题名: Product rotational polarization in photo-initiated bimolecular reactions A+BC: Dependence on the character of the potential energy surface for different mass combinations
作者: Wang, ML;  Han, KL;  He, GZ
刊名: JOURNAL OF PHYSICAL CHEMISTRY A
发表日期: 1998-12-10
卷: 102, 期:50, 页:10204-10210
收录类别: SCI
文章类型: Article
WOS标题词: Science & Technology ;  Physical Sciences
类目[WOS]: Chemistry, Physical ;  Physics, Atomic, Molecular & Chemical
研究领域[WOS]: Chemistry ;  Physics
英文摘要: In cases of light-heavy-light (LHL), light-light-heavy (LLH), and light-heavy-heavy (LHH) mass combinations, the product rotational polarization is reported using the quasiclassical trajectory method in the photoinitiated bimolecular reaction A + BC --> AB + C on attractive, mixed, and repulsive surfaces. Four polarization-dependent differential cross sections (PDDCS) which are sensitive to many photoinitiated bimolecular reaction experiments are presented. Furthermore, the dihedral angle distribution P(phi(r)) characterizing the K-K'-J' correlation and the distribution of angle between K and J' P(theta(r)) are discussed. Finally, the angular distributions P(theta(r),phi(r)) of product rotational vectors in the form of polar plots in theta(r) and phi(r) are shown.
关键词[WOS]: STATE-RESOLVED STEREODYNAMICS ;  CHEMILUMINESCENT REACTION ;  ANGULAR-CORRELATIONS ;  EXCHANGE-REACTIONS ;  CROSS-SECTIONS ;  ALIGNMENT ;  ORIENTATION ;  MOLECULES ;  DISTRIBUTIONS ;  MAGNITUDE
语种: 英语
WOS记录号: WOS:000077543700003
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/138465
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China

Recommended Citation:
Wang, ML,Han, KL,He, GZ. Product rotational polarization in photo-initiated bimolecular reactions A+BC: Dependence on the character of the potential energy surface for different mass combinations[J]. JOURNAL OF PHYSICAL CHEMISTRY A,1998,102(50):10204-10210.
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