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A novel catalytic approach to the production of aromatics and ethene directly from methane - (I) - Reaction process of methane on Mo/HZSM-5 catalyst
Wang, LS; Cui, W; Xu, YD; Guo, XX
关键词Methane Aromatics Ethene Mo/hzsm-5 Active Phase Tpsr
刊名PROGRESS IN NATURAL SCIENCE
1998-12-01
8期:6页:690-694
收录类别SCI
文章类型Article
WOS标题词Science & Technology ; Technology
类目[WOS]Materials Science, Multidisciplinary ; Multidisciplinary Sciences
研究领域[WOS]Materials Science ; Science & Technology - Other Topics
关键词[WOS]DEHYDRO-OLIGOMERIZATION ; BENZENE ; DEHYDROGENATION ; AROMATIZATION ; HYDROCARBONS
英文摘要The aromatization reaction of methane on Mo/HZSM-5 catalysts has been studied by temperature programmed surface reaction (TPSR) technique. Some oxygen-containing products, such as CO2, CO and H2O, were first produced. When these initial produces disappear, the contents of benzene and ethene in the effluent become maxima. It was suggested that during the initial stage a new active phase responsible for the transformation of methane into benzene and ethene may be formed through the redox interaction between methane and the Mo-containing catalyst. To form the active phase, Mo species should coexist with HZSM-5. The most active Mo/HZSM-5 catalyst was found to have the Mo loading between 2 %-3 %.
语种英语
WOS记录号WOS:000078714100006
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被引频次:1[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/138508
专题中国科学院大连化学物理研究所
作者单位Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China
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GB/T 7714
Wang, LS,Cui, W,Xu, YD,et al. A novel catalytic approach to the production of aromatics and ethene directly from methane - (I) - Reaction process of methane on Mo/HZSM-5 catalyst[J]. PROGRESS IN NATURAL SCIENCE,1998,8(6):690-694.
APA Wang, LS,Cui, W,Xu, YD,&Guo, XX.(1998).A novel catalytic approach to the production of aromatics and ethene directly from methane - (I) - Reaction process of methane on Mo/HZSM-5 catalyst.PROGRESS IN NATURAL SCIENCE,8(6),690-694.
MLA Wang, LS,et al."A novel catalytic approach to the production of aromatics and ethene directly from methane - (I) - Reaction process of methane on Mo/HZSM-5 catalyst".PROGRESS IN NATURAL SCIENCE 8.6(1998):690-694.
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