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Rotational state-to-state energy transfer of NH2((A)over-tilde(2)A(1)) in beam-gas condition
Dong, F; Li, XC; Zhang, M; Wang, XY; Lou, NQ
刊名JOURNAL OF CHEMICAL PHYSICS
1999-12-15
111期:23页:10578-10586
收录类别SCI
文章类型Article
WOS标题词Science & Technology ; Physical Sciences
类目[WOS]Physics, Atomic, Molecular & Chemical
研究领域[WOS]Physics
关键词[WOS]INTEGRAL CROSS-SECTIONS ; ANGULAR-MOMENTUM MODEL ; INELASTIC-SCATTERING ; MOLECULAR-COLLISIONS ; QUANTUM SCATTERING ; PROPENSITY RULES ; RATES ; OH
英文摘要The detailed study on the rotational state-to-state energy transfer (RSET) of NH2((A) over tilde (2)A(1)) at a relative translational energy of about 360 cm(-1) has been reported herein, by combining self-breakdown pulsed dc discharge and a photon counting technique. The transferred populations from the parent levels to the daughter levels have been obtained through the spectral simulations. It is clear that the rotational state distributions depend not only on the rotational quantum numbers of the initial and collisionally populated states, but also on the quantum number Ka. It is interesting to find that the probability of RSET behaves differently depending on the rotational quantum numbers of the parent levels, i.e., the exponential angular momentum transfer law (AMT) is preferred with the relatively low rotational levels, while the exponential energy gap law is preferred with the relatively high levels. According to the sudden approximation and the theory of Osborne , the experimental results are explained qualitatively. (C) 1999 American Institute of Physics. [S0021-9606(99)00247-0].
语种英语
WOS记录号WOS:000083927200024
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被引频次:5[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/138541
专题中国科学院大连化学物理研究所
作者单位Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China
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GB/T 7714
Dong, F,Li, XC,Zhang, M,et al. Rotational state-to-state energy transfer of NH2((A)over-tilde(2)A(1)) in beam-gas condition[J]. JOURNAL OF CHEMICAL PHYSICS,1999,111(23):10578-10586.
APA Dong, F,Li, XC,Zhang, M,Wang, XY,&Lou, NQ.(1999).Rotational state-to-state energy transfer of NH2((A)over-tilde(2)A(1)) in beam-gas condition.JOURNAL OF CHEMICAL PHYSICS,111(23),10578-10586.
MLA Dong, F,et al."Rotational state-to-state energy transfer of NH2((A)over-tilde(2)A(1)) in beam-gas condition".JOURNAL OF CHEMICAL PHYSICS 111.23(1999):10578-10586.
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