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题名: Applications of in situ NMR in catalytic processes of organic reactions
作者: Han, XW;  Yan, ZM;  Zhang, WP;  Bao, XH
刊名: CURRENT ORGANIC CHEMISTRY
发表日期: 2001-10-01
卷: 5, 期:10, 页:1017-1037
收录类别: SCI
文章类型: Review
WOS标题词: Science & Technology ;  Physical Sciences
类目[WOS]: Chemistry, Organic
研究领域[WOS]: Chemistry
英文摘要: In situ MAS NMR has been demonstrated to be a superior technique for analyzing desorbed reactants, reacting adsorbates, intermediates and products. The results are useful for getting deeper insights into catalytic processes and reaction kinetics, and for revealing the mechanisms of organic reactions. The utility of in situ NMR spectroscopy has demonstrated that this technique is an important means for the studies of catalytic organic reactions. The objective of this paper is to give a review on the generation of apparatus for in situ MAS NMR experiments, and to illustrate the applications of the in situ MAS NMR techniques in various important organic reactions catalyzed by solid catalysts. The typical reactions studied by in situ MAS NMR techniques include conversion of methanol to hydrocarbons (MTG process), aromatization of methane, ethylbenzene reaction over zeolite HMOR. observation of carbenium intermediates formation, and photocatalytic organic reaction.
关键词[WOS]: SOLID-STATE NMR ;  ANGLE-SPINNING NMR ;  METHANE DEHYDRO-AROMATIZATION ;  MOLECULAR-SIEVE CATALYSTS ;  TO-HYDROCARBON CHEMISTRY ;  CARBON CARBON BOND ;  PT-HMOR CATALYSTS ;  O-XYLENE MIXTURE ;  IN-SITU ;  MAS NMR
语种: 英语
WOS记录号: WOS:000172120000004
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/138848
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian, Peoples R China

Recommended Citation:
Han, XW,Yan, ZM,Zhang, WP,et al. Applications of in situ NMR in catalytic processes of organic reactions[J]. CURRENT ORGANIC CHEMISTRY,2001,5(10):1017-1037.
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