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题名: Non-Anderson-Schulz-Flory product distribution of Fischer-Tropsch synthesis over iron/activated charcoal catalyst
作者: Ma, WP;  Ding, YJ;  Luo, HY;  Lin, PZ;  Lin, LW
关键词: Fischer-Tropsch synthesis ;  iron ;  activated charcoal ;  supported catalyst ;  olefin ;  readsorption
刊名: CHINESE JOURNAL OF CATALYSIS
发表日期: 2001-05-01
卷: 22, 期:3, 页:279-282
收录类别: SCI
文章类型: Article
WOS标题词: Science & Technology ;  Physical Sciences ;  Technology
类目[WOS]: Chemistry, Applied ;  Chemistry, Physical ;  Engineering, Chemical
研究领域[WOS]: Chemistry ;  Engineering
英文摘要: The Fischer-Tropsch synthesis (FTS) product distribution and chain growth probability (Anderson-Schulz-Flory (ASF) chain growth probability and intrinsic chain growth probability) were studied on activated charcoal-supported iron (Fe/AC) catalyst in an autoclave slurry reactor. It was demonstrated that the product distribution on Fe/AC catalyst deviates from ASF product distribution. The experimental value at C-1 is larger than that in ASF product distribution, but the value at C-2 is lower than that in ASF plot. The chain growth investigation showed that the secondary reaction caused by olefins exists on Fe/AC catalyst under F-T condition, leading to that the product distribution deviates from ASF. It was showed that the water gas shift (WGS) reaction takes place simultaneously with FTS reaction. The XRD test found that there exist two kinds of active phases, FexC and Fe3O4, on the used Fe/AC catalyst.
关键词[WOS]: ALPHA-OLEFIN READSORPTION ;  IRON
语种: 英语
WOS记录号: WOS:000170359300018
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/138904
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China
2.Dalian Univ Technol, Dept Chem & Chem Engn, Dalian 116622, Peoples R China

Recommended Citation:
Ma, WP,Ding, YJ,Luo, HY,et al. Non-Anderson-Schulz-Flory product distribution of Fischer-Tropsch synthesis over iron/activated charcoal catalyst[J]. CHINESE JOURNAL OF CATALYSIS,2001,22(3):279-282.
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