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Further theoretical study of collisional quantum interference on rotational energy transfer in an atom diatom system
Tian, HM; Sun, MT; Sha, GH
刊名PHYSICAL CHEMISTRY CHEMICAL PHYSICS
2002
DOI10.1039/b205774c
4期:20页:5123-5127
收录类别SCI
文章类型Article
WOS标题词Science & Technology ; Physical Sciences
类目[WOS]Chemistry, Physical ; Physics, Atomic, Molecular & Chemical
研究领域[WOS]Chemistry ; Physics
关键词[WOS]TRIPLET MIXED STATES ; TRANSITIONS ; MOLECULES ; NA-2
英文摘要In our previous study (M.-T. Sun, G.-H. Sha, S.-L. Cong, F.-C. Ma, J.-C. Xie and C.-H. Zhang, Chem. Phys. Lett., 2001, 339, 413), a method of calculating the interference angle theoretically was presented, and experiments on the system CO A(1)Pi(v = 0) similar to e(3) Sigma(-)(v = 1) in collision with He were simulated. As a further theoretical study of the collision-induced quantum interference on rotational energy transfer in an atom diatom system, a dynamic model is described in this paper, based on the first order Born approximation of the time dependent perturbation theory and taking into account the anisotropic Lennard-Jones interaction potential. Experiments on the system CO A(1)Pi(v = 0) similar to e(3) Sigma(-) (v = 1) in collision with Ne and Ar in a sample cell are simulated. The integral interference phase angles are computed under both homonuclear and non-homonuclear approximations. The results are perfectly satisfactory under the latter condition.
语种英语
WOS记录号WOS:000178767800039
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被引频次:14[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/139074
专题中国科学院大连化学物理研究所
作者单位Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China
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Tian, HM,Sun, MT,Sha, GH. Further theoretical study of collisional quantum interference on rotational energy transfer in an atom diatom system[J]. PHYSICAL CHEMISTRY CHEMICAL PHYSICS,2002,4(20):5123-5127.
APA Tian, HM,Sun, MT,&Sha, GH.(2002).Further theoretical study of collisional quantum interference on rotational energy transfer in an atom diatom system.PHYSICAL CHEMISTRY CHEMICAL PHYSICS,4(20),5123-5127.
MLA Tian, HM,et al."Further theoretical study of collisional quantum interference on rotational energy transfer in an atom diatom system".PHYSICAL CHEMISTRY CHEMICAL PHYSICS 4.20(2002):5123-5127.
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