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题名: Further theoretical study of collisional quantum interference on rotational energy transfer in an atom diatom system
作者: Tian, HM;  Sun, MT;  Sha, GH
刊名: PHYSICAL CHEMISTRY CHEMICAL PHYSICS
发表日期: 2002
DOI: 10.1039/b205774c
卷: 4, 期:20, 页:5123-5127
收录类别: SCI
文章类型: Article
WOS标题词: Science & Technology ;  Physical Sciences
类目[WOS]: Chemistry, Physical ;  Physics, Atomic, Molecular & Chemical
研究领域[WOS]: Chemistry ;  Physics
英文摘要: In our previous study (M.-T. Sun, G.-H. Sha, S.-L. Cong, F.-C. Ma, J.-C. Xie and C.-H. Zhang, Chem. Phys. Lett., 2001, 339, 413), a method of calculating the interference angle theoretically was presented, and experiments on the system CO A(1)Pi(v = 0) similar to e(3) Sigma(-)(v = 1) in collision with He were simulated. As a further theoretical study of the collision-induced quantum interference on rotational energy transfer in an atom diatom system, a dynamic model is described in this paper, based on the first order Born approximation of the time dependent perturbation theory and taking into account the anisotropic Lennard-Jones interaction potential. Experiments on the system CO A(1)Pi(v = 0) similar to e(3) Sigma(-) (v = 1) in collision with Ne and Ar in a sample cell are simulated. The integral interference phase angles are computed under both homonuclear and non-homonuclear approximations. The results are perfectly satisfactory under the latter condition.
关键词[WOS]: TRIPLET MIXED STATES ;  TRANSITIONS ;  MOLECULES ;  NA-2
语种: 英语
WOS记录号: WOS:000178767800039
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/139074
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China

Recommended Citation:
Tian, HM,Sun, MT,Sha, GH. Further theoretical study of collisional quantum interference on rotational energy transfer in an atom diatom system[J]. PHYSICAL CHEMISTRY CHEMICAL PHYSICS,2002,4(20):5123-5127.
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