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题名: Femtosecond (2+1 ') pump-probe mass spectroscopy on the Rydberg states of ammonia
作者: Yin, SH;  Liu, HP;  Zhang, JY;  Jiang, B;  Xu, DL;  Wang, L;  Sha, GH;  Lou, NQ
刊名: CHEMICAL PHYSICS LETTERS
发表日期: 2002-04-22
卷: 356, 期:3-4, 页:227-232
收录类别: SCI
文章类型: Article
WOS标题词: Science & Technology ;  Physical Sciences
类目[WOS]: Chemistry, Physical ;  Physics, Atomic, Molecular & Chemical
研究领域[WOS]: Chemistry ;  Physics
英文摘要: The Rydberg state decay dynamics of ammonia is investigated in real-time by (2 + 1') femtosecond pump-probe ionization detection. The lifetime of ammonia in the (E) over tilde (1)A'(1) state is determined as 936 +/- 92 fs for the first time. The internal conversion (IC) pre-dissociation mechanism of the (E) over tilde'(1)A'(1), state has been discussed in this report. Concurrently, the (A) over tilde (1)A"(2) state (v'(2) = 4) lifetime is estimated as 51 +/- 4 fs, which is identical with the previous reports. (C) 2002 Elsevier Science B.V. All rights reserved.
关键词[WOS]: MULTIPHOTON IONIZATION SPECTROSCOPY ;  RESOLVED PHOTOELECTRON-SPECTROSCOPY ;  ULTRAFAST INTERNAL-CONVERSION ;  PHOTODISSOCIATION DYNAMICS ;  PREDISSOCIATION DYNAMICS ;  COOLED AMMONIA ;  EXCITED-STATES ;  BENZENE DIMER ;  MOLECULES ;  NH3
语种: 英语
WOS记录号: WOS:000175408600007
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/139091
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China

Recommended Citation:
Yin, SH,Liu, HP,Zhang, JY,et al. Femtosecond (2+1 ') pump-probe mass spectroscopy on the Rydberg states of ammonia[J]. CHEMICAL PHYSICS LETTERS,2002,356(3-4):227-232.
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