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Multiphoton ionization and ab initio calculation studies of pyridazine-(water)(n) clusters
Zhang, BL; Cai, Y; Mu, XL; Lou, NQ; Wang, XY
刊名CHEMICAL PHYSICS
2002-02-15
276期:3页:277-292
收录类别SCI
文章类型Article
WOS标题词Science & Technology ; Physical Sciences
类目[WOS]Chemistry, Physical ; Physics, Atomic, Molecular & Chemical
研究领域[WOS]Chemistry ; Physics
关键词[WOS]PHASE UNIMOLECULAR DECOMPOSITION ; DENSITY-FUNCTIONAL METHODS ; HYDROGEN-BONDED COMPLEXES ; PROTON-TRANSFER REACTIONS ; CARBON-DIOXIDE CLUSTERS ; GAS-PHASE ; AMMONIA CLUSTERS ; PHOTOELECTRON SPECTROSCOPY ; METASTABLE DECOMPOSITION ; BIOLOGICAL INTEREST
英文摘要The multiphoton ionization of the hydrogen-bonded clusters pyridazine-(water)(n) (C4H4N2-(H2O)(n)) was studied using a laser photoionization time-of-flight (TOF) mass spectrometer at the wavelengths of 355 and 532 nm. At both the wavelengths a series of protonated ions C4H4N2-(H2O)(n)H+ were observed. The results of ab initio calculations show that in the protonated products the proton prefers to link with the nitrogen atom. The dihedral angle formed by the water and pyridazine molecule planes is one of the important factors contributing to the stability of the binary cluster. The protonated. cluster ions measured in the experiment may be produced via an intracluster penning ionization or a charge transfer process. (C) 2002 Elsevier Science B.V. All rights reserved.
语种英语
WOS记录号WOS:000174013300005
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被引频次:11[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/139224
专题中国科学院大连化学物理研究所
作者单位Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China
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Zhang, BL,Cai, Y,Mu, XL,et al. Multiphoton ionization and ab initio calculation studies of pyridazine-(water)(n) clusters[J]. CHEMICAL PHYSICS,2002,276(3):277-292.
APA Zhang, BL,Cai, Y,Mu, XL,Lou, NQ,&Wang, XY.(2002).Multiphoton ionization and ab initio calculation studies of pyridazine-(water)(n) clusters.CHEMICAL PHYSICS,276(3),277-292.
MLA Zhang, BL,et al."Multiphoton ionization and ab initio calculation studies of pyridazine-(water)(n) clusters".CHEMICAL PHYSICS 276.3(2002):277-292.
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