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Quantum interference induced from the Lambda split of Pi state diatom
Li, YQ; Sun, MT; Ma, FC
关键词Collision-induced Rotational Energy Transfer Quantum Interference Cross Section Of Energy Transfer Transition Probability
刊名CHINESE JOURNAL OF CHEMICAL PHYSICS
2004-08-01
17期:4页:395-400
收录类别SCI
文章类型Article
WOS标题词Science & Technology ; Physical Sciences
类目[WOS]Physics, Atomic, Molecular & Chemical
研究领域[WOS]Physics
关键词[WOS]ROTATIONAL ENERGY-TRANSFER ; TRIPLET MIXED STATES ; ELECTRONIC STATES ; MOLECULES ; COLLISIONS ; SPECTROSCOPY ; TRANSITIONS ; REDUCTION ; SYSTEM ; NE
英文摘要To interpret theoretically the abnormal phenomenon in the experiment of collision-induced rotational energy transfer of CO (A (1)Pi, v = 3) with He by Sun et al., the time dependent first order Born approximation, and the long-range interaction potentials and "straight-line" trajectory approximation are taken into account. A theoretical model of quantum interference of II-state diatomic molecules, which originates from the difference between the two Lambda-related collision potential energy surfaces, is presented. The abnormal phenomenon of sigma(DeltaJ=0)(s-->s)<σ(s-->s)(&UDelta;J=+/-1) for He is also interpreted successfully. At first the theoretical development of collision-induced quantum interference on rotational energy transfer is reported; then a theoretical model of quantum interference of II-state diatomic molecules, which originates from the difference between the two A-related collision potential energy surfaces, is presented; in the end the results have been discussed and concluded.
语种英语
WOS记录号WOS:000223842300006
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被引频次:2[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/139393
专题中国科学院大连化学物理研究所
作者单位1.Liaoning Univ, Dept Phys, Shenyang 110036, Peoples R China
2.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol Raect Dynam, Dalian 116023, Peoples R China
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Li, YQ,Sun, MT,Ma, FC. Quantum interference induced from the Lambda split of Pi state diatom[J]. CHINESE JOURNAL OF CHEMICAL PHYSICS,2004,17(4):395-400.
APA Li, YQ,Sun, MT,&Ma, FC.(2004).Quantum interference induced from the Lambda split of Pi state diatom.CHINESE JOURNAL OF CHEMICAL PHYSICS,17(4),395-400.
MLA Li, YQ,et al."Quantum interference induced from the Lambda split of Pi state diatom".CHINESE JOURNAL OF CHEMICAL PHYSICS 17.4(2004):395-400.
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