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题名: A crossed molecular beam study on the dynamics of F atom reaction with SiH4
作者: Shen, Guanlin;  Yang, Xueming;  Shu, Jinian;  Yang, Chung-Hsin;  Lee, Yuan T.
刊名: JOURNAL OF CHEMICAL PHYSICS
发表日期: 2006-10-07
DOI: 10.1063/1.2217438
卷: 125, 期:13
收录类别: SCI
文章类型: Article
WOS标题词: Science & Technology ;  Physical Sciences
类目[WOS]: Physics, Atomic, Molecular & Chemical
研究领域[WOS]: Physics
英文摘要: In this report, the dynamics of the F+SiH4 reaction has been studied using the universal crossed molecular beam method. Angular resolved time-of-flight spectra have been measured for all reaction products in a single set of experiments. Two different reaction channels have been observed: HF+SiH3 and SiH3F+H. Product angular distributions as well as energy distributions were determined for these two product channels. Experimental results show that the HF product is forward scattered relative to the F atom beam direction, while the SiH3F product is backward scattered relative the F atom beam direction, suggesting that two reaction channels proceed with distinctive reaction dynamics. The relative branching ratios of the two channels have also been estimated. (c) 2006 American Institute of Physics.
关键词[WOS]: F+CD4 REACTION ;  F&H2 REACTION ;  SCATTERING ;  RESONANCES ;  PATHWAYS ;  SECTION
语种: 英语
WOS记录号: WOS:000241056600012
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/140260
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China
2.Chinese Acad Sci, Res Ctr Ecoenvironm Sci, Beijing 10085, Peoples R China
3.Acad Sinica, Inst Atom & Mol Sci, Taipei 106, Taiwan

Recommended Citation:
Shen, Guanlin,Yang, Xueming,Shu, Jinian,et al. A crossed molecular beam study on the dynamics of F atom reaction with SiH4[J]. JOURNAL OF CHEMICAL PHYSICS,2006,125(13).
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