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A crossed molecular beam study on the dynamics of F atom reaction with SiH4
Shen, Guanlin; Yang, Xueming; Shu, Jinian; Yang, Chung-Hsin; Lee, Yuan T.
刊名JOURNAL OF CHEMICAL PHYSICS
2006-10-07
DOI10.1063/1.2217438
125期:13
收录类别SCI
文章类型Article
WOS标题词Science & Technology ; Physical Sciences
类目[WOS]Physics, Atomic, Molecular & Chemical
研究领域[WOS]Physics
关键词[WOS]F+CD4 REACTION ; F&H2 REACTION ; SCATTERING ; RESONANCES ; PATHWAYS ; SECTION
英文摘要In this report, the dynamics of the F+SiH4 reaction has been studied using the universal crossed molecular beam method. Angular resolved time-of-flight spectra have been measured for all reaction products in a single set of experiments. Two different reaction channels have been observed: HF+SiH3 and SiH3F+H. Product angular distributions as well as energy distributions were determined for these two product channels. Experimental results show that the HF product is forward scattered relative to the F atom beam direction, while the SiH3F product is backward scattered relative the F atom beam direction, suggesting that two reaction channels proceed with distinctive reaction dynamics. The relative branching ratios of the two channels have also been estimated. (c) 2006 American Institute of Physics.
语种英语
WOS记录号WOS:000241056600012
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被引频次:7[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/140260
专题中国科学院大连化学物理研究所
作者单位1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China
2.Chinese Acad Sci, Res Ctr Ecoenvironm Sci, Beijing 10085, Peoples R China
3.Acad Sinica, Inst Atom & Mol Sci, Taipei 106, Taiwan
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Shen, Guanlin,Yang, Xueming,Shu, Jinian,et al. A crossed molecular beam study on the dynamics of F atom reaction with SiH4[J]. JOURNAL OF CHEMICAL PHYSICS,2006,125(13).
APA Shen, Guanlin,Yang, Xueming,Shu, Jinian,Yang, Chung-Hsin,&Lee, Yuan T..(2006).A crossed molecular beam study on the dynamics of F atom reaction with SiH4.JOURNAL OF CHEMICAL PHYSICS,125(13).
MLA Shen, Guanlin,et al."A crossed molecular beam study on the dynamics of F atom reaction with SiH4".JOURNAL OF CHEMICAL PHYSICS 125.13(2006).
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