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Quantitative measurement and interpretation of optical second harmonic generation from molecular interfaces
Zhang, Wen-kai; Wang, Hong-fei; Zheng, De-sheng
Source PublicationPHYSICAL CHEMISTRY CHEMICAL PHYSICS
2006
DOI10.1039/b608005g
Volume8Issue:35Pages:4041-4052
Indexed BySCI
SubtypeReview
WOS HeadingsScience & Technology ; Physical Sciences
WOS SubjectChemistry, Physical ; Physics, Atomic, Molecular & Chemical
WOS Research AreaChemistry ; Physics
WOS Keyword2ND HARMONIC-GENERATION ; SUM-FREQUENCY GENERATION ; ORIENTATION-INSENSITIVE METHODOLOGY ; SURFACE VIBRATIONAL SPECTROSCOPY ; SELF-ASSEMBLED MONOLAYERS ; LANGMUIR-BLODGETT-FILMS ; AIR-WATER-INTERFACE ; MULTIPOLAR CONTRIBUTIONS ; AIR/WATER INTERFACE ; ISOTROPIC FLUIDS
AbstractSecond harmonic generation (SHG) has been proven a uniquely effective technique in the investigation of molecular structure and conformations, as well as dynamics of molecular interfaces. The ability to apply SHG to molecular interface studies depends on the ability to abstract quantitative information from the measurable quantities in the actual SHG experiments. In this review, we try to assess recent developments in the SHG experimental methodologies towards quantitative analysis of the nonlinear optical properties of the achiral molecular interfaces with rotational isotropy along the interface normal. These developments include the methodology for orientational analysis of the SHG experimental data, the experimental approaches for more accurate SHG measurements, and a novel treatment of the symmetry properties of the molecular polarizability tensors in association with the experimentally measurable quantities. In the end, the recent developments on the problem of surface versus bulk contribution in SHG surface studies is discussed. These developments can put SHG on a more solid foundation for molecular interface studies, and to pave the way for better understanding and application of SHG surface studies in general.
Language英语
WOS IDWOS:000240109300001
Citation statistics
Cited Times:50[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/140330
Collection中国科学院大连化学物理研究所
Affiliation1.Chinese Acad Sci, Inst Chem, State Key Lab Mol React Dynam, Beijing 100080, Peoples R China
2.Grad Univ Chinese Acad Sci, Beijing 100864, Peoples R China
Recommended Citation
GB/T 7714
Zhang, Wen-kai,Wang, Hong-fei,Zheng, De-sheng. Quantitative measurement and interpretation of optical second harmonic generation from molecular interfaces[J]. PHYSICAL CHEMISTRY CHEMICAL PHYSICS,2006,8(35):4041-4052.
APA Zhang, Wen-kai,Wang, Hong-fei,&Zheng, De-sheng.(2006).Quantitative measurement and interpretation of optical second harmonic generation from molecular interfaces.PHYSICAL CHEMISTRY CHEMICAL PHYSICS,8(35),4041-4052.
MLA Zhang, Wen-kai,et al."Quantitative measurement and interpretation of optical second harmonic generation from molecular interfaces".PHYSICAL CHEMISTRY CHEMICAL PHYSICS 8.35(2006):4041-4052.
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