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题名: Transfer dehydrogenation of alcohols over ceria-supported Cu, Ir, and Pd catalysts
作者: Song Wei;  Shi Ruijuan;  Liu Junlong;  Zhan Ensheng;  Li Zhanshuang;  Xu Yide;  Shen Wenjie
关键词: copper ;  iridium ;  palladium ;  ceria ;  alcohol ;  transfer dehydrogenation
刊名: CHINESE JOURNAL OF CATALYSIS
发表日期: 2007-02-01
卷: 28, 期:2, 页:106-108
收录类别: SCI
文章类型: Article
WOS标题词: Science & Technology ;  Physical Sciences ;  Technology
类目[WOS]: Chemistry, Applied ;  Chemistry, Physical ;  Engineering, Chemical
研究领域[WOS]: Chemistry ;  Engineering
英文摘要: Ceria-supported Cu, Ir, and Pd catalysts showed quite promising activity for transfer dehydrogenation of cyclohexanol and 2-octanol to cyclohexanone and 2-octanone, respectively, using styrene as the hydrogen acceptor. The Cu/CeO2 and Pd/CeO2 catalysts were more active than the previously reported Cu and Pd catalysts supported on Al2O3, and Ir/CeO2 exhibited extremely high activity. The reactivity of alcohols decreased in the order 2-octanol > cyclohexanol > benzyl alcohol > 1-octanol. The synergetic effect between the metals and CeO2 as well as the effective coupling of dehydrogenation of alcohols and hydrogenation of styrene was responsible for the high catalytic activity.
关键词[WOS]: TRANSFER HYDROGENATION ;  SELECTIVE OXIDATION ;  METAL-CATALYSTS ;  OXYGEN
语种: 英语
WOS记录号: WOS:000244994000004
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/140602
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Harbin Engn Univ, Coll Mat Sci & Chem Engn, Harbin 150001, Heilongjiang, Peoples R China
2.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China

Recommended Citation:
Song Wei,Shi Ruijuan,Liu Junlong,et al. Transfer dehydrogenation of alcohols over ceria-supported Cu, Ir, and Pd catalysts[J]. CHINESE JOURNAL OF CATALYSIS,2007,28(2):106-108.
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