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题名: Experimental observables and macroscopic Susceptibility/Microscopic polarizability tensors for third and fourth-order Nonlinear Spectroscopy of ordered molecular system
作者: Wang, Yuan;  Cui, Zhi-Feng;  Wang, Hong-Fei
关键词: third and fourth-order nonlinear spectroscopy ;  experimental observable ;  macroscopic susceptibility/microscopic polarizability tenser ;  ordered molecular system
刊名: CHINESE JOURNAL OF CHEMICAL PHYSICS
发表日期: 2007-08-27
DOI: 10.1088/1674-0068/20/04/449-460
卷: 20, 期:4, 页:449-460
收录类别: SCI
文章类型: Article
WOS标题词: Science & Technology ;  Physical Sciences
类目[WOS]: Physics, Atomic, Molecular & Chemical
研究领域[WOS]: Physics
英文摘要: There has been emerging needs for the quantitative polarization analysis for the Coherent Anti-stakes Raman Spectroscopy and Coherent Anti-stokes Hyper-raman Spectroscopy, as the experimental studies with coherent anti-stokes raman spectroscopy and coherent anti-stokes hyper-raman spectroscopy for the interface and membrane studies being growing. Recently we have demonstrated that orientational analysis of linear and nonlinear spectroscopy from the ordered molecular system, such as molecular interfaces and films, can be carried out with the formulation of the orientational function in simple functional forms. Applications of such formulation for the second order spectroscopy, namely, the Second Harmonic Generation and Sum Frequency Generation Vibrational Spectroscopy, have helped to understand spectral and orientational details of the molecular interfaces and films. In order to employ this formulation for the higher order coherent nonlinear spectroscopy, the detailed expressions of the experimental observables and the macroscopic susceptibility/microscopic polarizability tensors for the third and fourth-order nonlinear spectroscopy for the interface or film is presented with the rotational symmetry. General expressions for the typical third and fourth order spectroscopy, such as the Third Harmonic Generation, the degenerated coherent anti-stokes raman spectroscopy, the Fourth Harmonic Generation and the degenerated coherent anti-stokes hyper-raman spectroscopy, are presented for their future applications. The advantages and limitations of the third and fourth order spectroscopic techniques are also discussed.
关键词[WOS]: SUM-FREQUENCY GENERATION ;  STOKES-RAMAN SCATTERING ;  SURFACE-ADSORPTION LAYERS ;  CH STRETCHING MODES ;  VIBRATIONAL SPECTROSCOPY ;  PARAMETRIC-AMPLIFICATION ;  2ND-HARMONIC GENERATION ;  LIQUID INTERFACE ;  WATER-MOLECULES ;  METHYL-GROUP
语种: 英语
WOS记录号: WOS:000249465100020
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/140732
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Anhui Normal Univ, Dept Phys, Wuhu 241000, Peoples R China
2.Chinese Acad Sci, Inst Chem, State Key Lab Mol React Dynam, Beijing 100080, Peoples R China

Recommended Citation:
Wang, Yuan,Cui, Zhi-Feng,Wang, Hong-Fei. Experimental observables and macroscopic Susceptibility/Microscopic polarizability tensors for third and fourth-order Nonlinear Spectroscopy of ordered molecular system[J]. CHINESE JOURNAL OF CHEMICAL PHYSICS,2007,20(4):449-460.
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