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Base-base bifunctional catalysis: A practical strategy for asymmetric Michael addition of malonates to alpha,beta-unsaturated aldehydes
Wang, Yongcan1; Li, Pengfei1; Liang, Xinmiao1,2; Ye, Jinxing1,2
关键词Aldehydes Asymmetric Catalysis Bifunctional Catalysis Malonates Michael Addition
刊名ADVANCED SYNTHESIS & CATALYSIS
2008-06-01
DOI10.1002/adsc.200800070
350期:9页:1383-1389
收录类别SCI ; IC ; CCR
文章类型Article
WOS标题词Science & Technology ; Physical Sciences
类目[WOS]Chemistry, Applied ; Chemistry, Organic
研究领域[WOS]Chemistry
关键词[WOS]ORGANOCATALYTIC CONJUGATE ADDITION ; ENANTIOSELECTIVE MICHAEL ; CINCHONA ALKALOIDS ; ORGANIC CATALYSIS ; IMINIUM CATALYSIS ; MANNICH REACTION ; C-C ; PROLINE ; DERIVATIVES ; ALDOL
英文摘要Lewis base-Bronsted base bifunctional catalysis is a novel and practical strategy for the asymmetric Michael addition. The addition of malonates to a series of cc,p-unsaturated aldehydes can take place under base-base bifunctional catalytic conditions using 0.5-5 mol% of (S)-2-[diphenyl(trimethyl-silyloxy)methyl]pyrrolidine as catalyst and 5-30 mol% of lithium 4-fluorobenzoate as additive base with up to 99% ee.
语种英语
WOS记录号WOS:000256976100031
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被引频次:44[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/140928
专题中国科学院大连化学物理研究所
作者单位1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China
2.E China Univ Sci & Technol, Sch Pharm, Minist Educ, Engn Res Ctr Pharmaceut Proc Chem, Shanghai 200237, Peoples R China
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GB/T 7714
Wang, Yongcan,Li, Pengfei,Liang, Xinmiao,et al. Base-base bifunctional catalysis: A practical strategy for asymmetric Michael addition of malonates to alpha,beta-unsaturated aldehydes[J]. ADVANCED SYNTHESIS & CATALYSIS,2008,350(9):1383-1389.
APA Wang, Yongcan,Li, Pengfei,Liang, Xinmiao,&Ye, Jinxing.(2008).Base-base bifunctional catalysis: A practical strategy for asymmetric Michael addition of malonates to alpha,beta-unsaturated aldehydes.ADVANCED SYNTHESIS & CATALYSIS,350(9),1383-1389.
MLA Wang, Yongcan,et al."Base-base bifunctional catalysis: A practical strategy for asymmetric Michael addition of malonates to alpha,beta-unsaturated aldehydes".ADVANCED SYNTHESIS & CATALYSIS 350.9(2008):1383-1389.
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